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Ultrastrongly Coupled Exciton–Polaritons in Metal‐Clad Organic Semiconductor Microcavities
Abstract
Ultrastrong exciton–photon coupling of Frenkel molecular excitons is demonstrated at room temperature in a metal‐clad microcavity containing a thin film of 2,7‐bis[9,9‐di(4‐methylphenyl)‐fluoren‐2‐yl]‐9,9‐di(4‐methylphenyl)fluorene. A giant Rabi splitting of Ω ∼ 1 eV is measured using angle‐resolved reflectivity and bright photoluminescence is observed from the lower polariton branch. To obtain the virtual photon and exciton content of the polariton ground state, the results are interpreted in terms of the full Hopfield Hamiltonian, including anti‐resonant terms. Also included is an analytical treatment of the often ignored and sometimes misinterpreted TM‐polarized metal–insulator–metal plasmon–polariton.
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Citations
Cites
Room-Temperature Polariton Lasing in an Organic Single-Crystal Microcavity
Kéna-Cohen, S., & Forrest, S. R. (2010) · Nature Photonics · doi:10.1038/nphoton.2010.86 · Cited by 942
Cited by
Microwave photonics with superconducting quantum circuits
Gu, X., Kockum, A. F., Miranowicz, A., Liu, Y.-X., & Nori, F. (2017) · Physics Reports · doi:10.1016/j.physrep.2017.10.002 · Cited by 1,307
Nonlinear Interactions in an Organic Polariton Condensate
Daskalakis, K. S., Maier, S. A., Murray, R., & Kéna-Cohen, S. (2014) · Nature Materials · doi:10.1038/nmat3874 · Cited by 484
Self-citationPolaritonic Chemistry with Organic Molecules
Feist, J., Galego, J., & Garcia-Vidal, F. J. (2018) · ACS Photonics · doi:10.1021/acsphotonics.7b00680 · Cited by 438
Grant, R. T., Michetti, P., Musser, A. J., Gregoire, P., Virgili, T., Vella, E., Cavazzini, M., Georgiou, K., Galeotti, F., Clark, C., et al. (2016) · Advanced Optical Materials · doi:10.1002/adom.201600337 · Cited by 100
Metadata
- Authors
- Kéna‐Cohen, S., Maier, S. A., & Bradley, D. D. C.
- Venue
- Advanced Optical Materials
- Publisher
- Wiley
- Published
- 2013-08-05
- Volume
- 1
- Issue
- 11
- Pages
- 827-833
- ISSN
- 2195-1071 (ISSN-L)
- OpenAlex
- W2057090058
- Cited by
- 231
- References
- 1
- FWCI
- 6.68
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kéna‐Cohen, S., Maier, S. A., & Bradley, D. D. C. (2013). Ultrastrongly Coupled Exciton–Polaritons in Metal‐Clad Organic Semiconductor Microcavities. Advanced Optical Materials. https://doi.org/10.1002/adom.201300256
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