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High Performance Solid Polymer Electrolytes for Rechargeable Batteries: A Self‐Catalyzed Strategy toward Facile Synthesis
Open accessAbstract
It is urgent to seek high performance solid polymer electrolytes (SPEs) via a facile chemistry and simple process. The lithium salts are composed of complex anions that are stabilized by a Lewis acid agent. This Lewis acid can initiate the ring opening polymerization. Herein, a self‐catalyzed strategy toward facile synthesis of crosslinked poly(ethylene glycol) diglycidyl ether‐based solid polymer electrolyte (C‐PEGDE) is presented. It is manifested that the poly(ethylene glycol) diglycidyl ether‐based solid polymer electrolyte possesses a superior electrochemical stability window up to 4.5 V versus Li/Li+ and considerable ionic conductivity of 8.9 × 10−5 S cm−1 at ambient temperature. Moreover, the LiFePO 4/C‐PEGDE/Li batteries deliver stable charge/discharge profiles and considerable rate capability. It is demonstrated that this self‐catalyzed strategy can be a very effective approach for high performance solid polymer electrolytes.
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Cites
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Ring-Opening Polymerization—An Introductory Review
Nuyken, O., & Pask, S. (2013) · Polymers · doi:10.3390/polym5020361 · Cited by 456
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Reducing the thickness of solid-state electrolyte membranes for high-energy lithium batteries
Wu, J., Yuan, L., Zhang, W., Li, Z., Xie, X., & Huang, Y. (2021) · Energy & Environmental Science · doi:10.1039/d0ee02241a · Cited by 425
Lithium anode stable in air for low-cost fabrication of a dendrite-free lithium battery
Shen, X., Li, Y., Qian, T., Liu, J., Zhou, J., Yan, C., & Goodenough, J. B. (2019) · Nature Communications · doi:10.1038/s41467-019-08767-0 · Cited by 386
In situ polymerization process: an essential design tool for lithium polymer batteries
Vijayakumar, V., Anothumakkool, B., Kurungot, S., Winter, M., & Nair, J. R. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03527k · Cited by 365
Progress in Solid Polymer Electrolytes for Lithium‐Ion Batteries and Beyond
An, Y., Han, X., Liu, Y., Azhar, A., Na, J., Nanjundan, A. K., Wang, S., Yu, J., & Yamauchi, Y. (2022) · Small · doi:10.1002/smll.202103617 · Cited by 363
Metadata
- Authors
- Cui, Y., Liang, X., Chai, J., Cui, Z., Wang, Q., He, W., Liu, X., Liu, Z., Cui, G., & Feng, J.
- Venue
- Advanced Science
- Publisher
- Wiley
- Published
- 2017-08-02
- Volume
- 4
- Issue
- 11
- Pages
- 1700174-1700174
- ISSN
- 2198-3844 (ISSN-L)
- OpenAlex
- W2742936675
- Cited by
- 210
- References
- 2
- FWCI
- 7.94
- Type
- journal article
- Language
- en
- Open access
- gold
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- Cui, Y., Liang, X., Chai, J., Cui, Z., Wang, Q., He, W., Liu, X., Liu, Z., Cui, G., & Feng, J. (2017). High Performance Solid Polymer Electrolytes for Rechargeable Batteries: A Self‐Catalyzed Strategy toward Facile Synthesis. Advanced Science. https://doi.org/10.1002/advs.201700174
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