Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges

Pan, Hu; Li, Jinglin; Wang, Yangang; Xia, Qineng; Qiu, Liang; Zhou, Baowen

doi:10.1002/advs.202402651

Cited by 67Advanced Photocatalysis TechniquesCatalysis for Biomass ConversionThermochemical Biomass Conversion Processes

Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges

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Pan, Hu, Li, Jinglin, Wang, Yangang, Xia, Qineng, Qiu, Liang, Zhou, Baowen·2024·Advanced Science

DOI 10.1002/advs.202402651PMC PMC11304308

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Abstract

Hydrogen (H 2) has emerged as a clean and versatile energy carrier to power a carbon‐neutral economy for the post‐fossil era. Hydrogen generation from low‐cost and renewable biomass by virtually inexhaustible solar energy presents an innovative strategy to process organic solid waste, combat the energy crisis, and achieve carbon neutrality. Herein, the progress and breakthroughs in solar‐powered H 2 production from biomass are reviewed. The basic principles of solar‐driven H 2 generation from biomass are first introduced for a better understanding of the reaction mechanism. Next, the merits and shortcomings of various semiconductors and cocatalysts are summarized, and the strategies for addressing the related issues are also elaborated. Then, various bio‐based feedstocks for solar‐driven H 2 production are reviewed with an emphasis on the effect of photocatalysts and catalytic systems on performance. Of note, the concurrent generation of value‐added chemicals from biomass reforming is emphasized as well. Meanwhile, the emerging photo‐thermal coupling strategy that shows a grand prospect for maximally utilizing the entire solar energy spectrum is also discussed. Further, the direct utilization of hydrogen from biomass as a green reductant for producing value‐added chemicals via organic reactions is also highlighted. Finally, the challenges and perspectives of photoreforming biomass toward hydrogen are envisioned.

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Authors: Pan, H., Li, J., Wang, Y., Xia, Q., Qiu, L., & Zhou, B.
Affiliations: College of Biological Chemical Science and Engineering Jiaxing University 899 Guangqiong Road Jiaxing Zhejiang 314001 China
Shanghai Jiao Tong University (CN)
Jiaxing University (CN)
Corresponding author: Wang, Yangang
Zhou, Baowen
ORCID: Li, Jinglin
Wang, Yangang
Xia, Qineng
Zhou, Baowen
Venue: Advanced Science
Publisher: Wiley
Published: 2024-05-30
Volume: 11
Issue: 29
Pages: e2402651-e2402651
ISSN: 2198-3844 (ISSN-L)
DOI: 10.1002/advs.202402651
PMC: PMC11304308
OpenAlex: W4399246574
Cited by: 67
References: 350
Citations by year: 2026: 26 · 2025: 32 · 2024: 9
FWCI: 1.40
Type: journal article
Language: en
Open access: gold
doi.org
Licence: cc-by
creativecommons.org/licenses/by/4.0/ (vor)
Locations: Advanced Science (publishedVersion, cc-by)
PubMed Central (publishedVersion, cc-by)
PubMed (publishedVersion)
DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
Funders: Natural Science Foundation of Zhejiang Province (LQ22B060008)
National Natural Science Foundation of China (22109095, 22278176)
National Key Research and Development Program of China (2023YFB4004900)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
Physical Sciences › Engineering › Biomedical Engineering › Catalysis for Biomass Conversion
Physical Sciences › Engineering › Biomedical Engineering › Thermochemical Biomass Conversion Processes
Keywords: solar hydrogen production, photocatalytic hydrogen evolution, semiconductors, cocatalyst, bio-based feedstocks, value-added chemicals, organic reactions, carbon neutrality, organic solid waste

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Solar‐Driven Biomass Reforming for Hydrogen Generation: Principles, Advances, and Challenges

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