The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Vacancy Engineering for Tuning Electron and Phonon Structures of Two‐Dimensional Materials
Abstract
2D inorganic materials are now breeding a wide‐ranging series of energy applications including catalysis, electrochemical activity, thermoelectricity and spin electronic devices. However, the physicochemical property of virgin 2D inorganic materials can scarcely satisfy the modern increasing diversificated demand of theory and applcations. In this regard, confined electron and phonon structures will be a directive for rationally tuning the intrinsic properties of 2D inorganic materials. Given this, vacancies in even infinitesimal concentrations could unlock the huge potential that exists for manipulating the energy band structure, carrier concentration, spin nature and phonon vibration and migration, which in turn will lead to the functionalization of intrinsic properties, particular in atom‐thick 2D solids. The concept of vacancy regulation embodies the design philosophy of “less is more”, and provides an opportunity to explore uncharted quantum phenomenon. In this review, recent progress in the design of appropriate vacancies on the 2D plane, particularly from the authors' own laboratories, is summarized, and the vacancy regulation rules of electron and phonon behavior are explained. Finally, based on an unambiguous understanding of the structure–property relationships between the vacancy, electron‐phonon behavior, and the intrinsic properties, future possibilities for the rational design of vacancies to acquire desirable properties are explored.
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Cites
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
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Self-citationTwo-dimensional transition metal dichalcogenide nanosheet-based composites
Tan, C., & Zhang, H. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00182f · Cited by 1,605
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Self-citationLow Overpotential in Vacancy-Rich Ultrathin CoSe2 Nanosheets for Water Oxidation
Liu, Y., Cheng, H., Lyu, M., Fan, S., Liu, Q., Zhang, W., Zhi, Y., Wang, C., Xiao, C., Wei, S., et al. (2014) · Journal of the American Chemical Society · doi:10.1021/ja5085157 · Cited by 1,094
Self-citationGeneration and electric control of spin–valley-coupled circular photogalvanic current in WSe2
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Cited by
Xiao, Z., Huang, Y.-C., Dong, C.-L., Xie, C., Liu, Z., Du, S., Chen, W., Yan, D., Tao, L., Shu, Z., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00257 · Cited by 1,445
Oxygen Vacancy‐Mediated Photocatalysis of BiOCl: Reactivity, Selectivity, and Perspectives
Li, H., Li, J., Ai, Z., Jia, F., & Zhang, L. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201705628 · Cited by 1,207
Zhang, S., Liu, X., Liu, C., Luo, S., Wang, L., Cai, T., Zeng, Y., Yuan, J., Dong, W., Pei, Y., et al. (2018) · ACS Nano · doi:10.1021/acsnano.7b07974 · Cited by 709
Self-citationDefect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
Oxygen‐Vacancy Abundant Ultrafine Co3O4/Graphene Composites for High‐Rate Supercapacitor Electrodes
Yang, S., Liu, Y., Hao, Y., Yang, X., Goddard, W. A., Zhang, X. L., & Cao, B. (2018) · Advanced Science · doi:10.1002/advs.201700659 · Cited by 498
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Metadata
- Authors
- Liu, Y., Xiao, C., Li, Z., & Xie, Y.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2016-08-22
- Volume
- 6
- Issue
- 23
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2507314349
- Cited by
- 275
- References
- 7
- FWCI
- 11.64
- Type
- journal article
- Language
- en
- Open access
- closed
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