The DOI matches its Crossref record; 24 of the 24 references it cites were found in a registry or an index.
Engineering Local Coordination Environments of Atomically Dispersed and Heteroatom‐Coordinated Single Metal Site Electrocatalysts for Clean Energy‐Conversion
Abstract
Carbon‐based heteroatom‐coordinated single‐atom catalysts (SACs) are promising candidates for energy‐related electrocatalysts because of their low‐cost, tunable catalytic activity/selectivity, and relatively homogeneous morphologies. Unique interactions between single metal sites and their surrounding coordination environments play a significant role in modulating the electronic structure of the metal centers, leading to unusual scaling relationships, new reaction mechanisms, and improved catalytic performance. This review summarizes recent advancements in engineering of the local coordination environment of SACs for improved electrocatalytic performance for several crucial energy‐convention electrochemical reactions: oxygen reduction reaction, hydrogen evolution reaction, oxygen evolution reaction, CO 2 reduction reaction, and nitrogen reduction reaction. Various engineering strategies including heteroatom‐doping, changing the location of SACs on their support, introducing external ligands, and constructing dual metal sites are comprehensively discussed. The controllable synthetic methods and the activity enhancement mechanism of state‐of‐the‐art SACs are also highlighted. Recent achievements in the electronic modification of SACs will provide an understanding of the structure–activity relationship for the rational design of advanced electrocatalysts.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
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High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
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Self-citationAtomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
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Platinum single-atom and cluster catalysis of the hydrogen evolution reaction
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Atomic cobalt on nitrogen-doped graphene for hydrogen generation
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Cited by
Liu, S., Li, C., Zachman, M. J., Zeng, Y., Yu, H., Li, B., Wang, M., Braaten, J., Liu, J., Meyer, H. M., et al. (2022) · Nature Energy · doi:10.1038/s41560-022-01062-1 · Cited by 733
Self-citationRecent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Metadata
- Authors
- Zhu, Y., Sokolowski, J., Song, X., He, Y., Mei, Y., & Wu, G.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2019-12-20
- Volume
- 10
- Issue
- 11
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2995257855
- Cited by
- 392
- References
- 24
- FWCI
- 10.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhu, Y., Sokolowski, J., Song, X., He, Y., Mei, Y., & Wu, G. (2020). Engineering Local Coordination Environments of Atomically Dispersed and Heteroatom‐Coordinated Single Metal Site Electrocatalysts for Clean Energy‐Conversion. Advanced Energy Materials. https://doi.org/10.1002/aenm.201902844
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