The DOI matches its Crossref record; 14 of the 14 references it cites were found in a registry or an index.
Molecular Design of Single‐Atom Catalysts for Oxygen Reduction Reaction
Abstract
Fuel cells are highly attractive for direct chemical‐to‐electrical energy conversion and represent the ultimate mobile power supply solution. However, presently, fuel cells are limited by the sluggish kinetics of the cathodic oxygen reduction reaction (ORR), which requires the use of Pt as a catalyst, thus significantly increasing the overall cost of the cells. Recently, nonprecious metal single‐atom catalysts (SACs) with high ORR activity under both acidic and alkaline conditions have been recognized as promising cost‐effective alternatives to replace Pt in fuel cells. Considerable efforts have been devoted to further improving the ORR activity of SACs, including tailoring the coordination structure of the metal centers, enriching the concentration of the metal centers, and engineering the electronic structure and porosity of the substrate. Herein, a brief introduction to fuel cells and fundamentals of the ORR parameters of SACs and the origin of their high activity is provided, followed by a detailed review of the recently developed strategies used to optimize the ORR activity of SACs in both rotating disk electrode and membrane electrode assembly tests. Remarks and perspectives on the remaining challenges and future directions of SACs for the development of commercial fuel cells are also presented.
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Combining theory and experiment in electrocatalysis: Insights into materials design
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Cited by
Boosting Oxygen Electrocatalytic Activity of Fe–N–C Catalysts by Phosphorus Incorporation
Zhou, Y., Lu, R., Tao, X., Qiu, Z., Chen, G., Yang, J., Zhao, Y., Feng, X., & Müllen, K. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.2c12933 · Cited by 567
Recent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Palladium alloys used as electrocatalysts for the oxygen reduction reaction
Wang, T., Chutia, A., Brett, D. J. L., Shearing, P. R., He, G., Chai, G., & Parkin, I. P. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03915b · Cited by 322
Hu, X., Chen, S., Chen, L., Tian, Y., Yao, S., Lu, Z., Zhang, X., & Zhou, Z. (2022) · Journal of the American Chemical Society · doi:10.1021/jacs.2c08743 · Cited by 322
Application of Molecular Catalysts for the Oxygen Reduction Reaction in Alkaline Fuel Cells
Friedman, A., Mizrahi, M., Levy, N., Zion, N., Zachman, M., & Elbaz, L. (2021) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.1c16311 · Cited by 42
Metadata
- Authors
- Wan, C., Duan, X., & Huang, Y.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2020-02-25
- Volume
- 10
- Issue
- 14
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W3008313783
- Cited by
- 439
- References
- 14
- FWCI
- 13.92
- Type
- journal article
- Language
- en
- Open access
- closed
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