The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Structural Regulation and Support Coupling Effect of Single‐Atom Catalysts for Heterogeneous Catalysis
Abstract
Single atom catalysts (SACs) that integrate the merits of homogeneous and heterogeneous catalysts have been attracting considerable attention in recent years. The individual metal atoms of SACs can be stabilized on supports through various unsaturated chemical sites or space confinement for achieving the maximized atom utilization efficiency. Aside from the development of strategies for preparing high loading and high purity SACs, another key challenge in this field is precisely manipulating the geometric and electronic structure of catalytically active single metal sites, thus rendering the catalysts exceptionally reactive, selective, and stabile compared to their bulk counterparts. This review summarizes recent advancements in SACs for heterogeneous catalysis from the perspective of local structural regulation and the synergistic coupling effect between metal species and supports. Special emphasis is placed on the elucidation of the catalytic structure‐performance relationship in terms of coordination environment, valence state and metal‐support interactions by advanced characterization and theoretical studies. Select in situ or operando characterization techniques for tracking the SACs’ structure evolution under realistic conditions are highlighted. Finally, the challenges and opportunities are discussed to offer insight into the rational design of more intriguing SACs with high activity and distinct chemoselectivity.
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Cites
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Self-citationAnchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
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Cited by
Song, H., Wu, M., Tang, Z., Tse, J. S., Yang, B., & Lu, S. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202017102 · Cited by 508
Wang, Y., Liu, Y., Liu, W., Wu, J., Li, Q., Feng, Q., Chen, Z., Xiong, X., Wang, D., & Lei, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02833a · Cited by 303
Qiu, Y., Liu, S., Wei, C., Fan, J., Yao, H., Dai, L., Wang, G., Li, H., Su, B., & Guo, X. (2022) · Chemical Engineering Journal · doi:10.1016/j.cej.2021.131309 · Cited by 93
Metadata
- Authors
- Liu, D., He, Q., Ding, S., & Song, L.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2020-07-14
- Volume
- 10
- Issue
- 32
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W3042628747
- Cited by
- 307
- References
- 10
- FWCI
- 15.20
- Type
- journal article
- Language
- en
- Open access
- closed
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