The DOI matches its Crossref record.
Ein stabiler “Single‐site”‐Palladiumkatalysator für Hydrierungen
Abstract
Wir beschreiben die Herstellung und das Hydrierungsverhalten eines Einzelatom‐Palladiumkatalysators, geschaffen durch die Verankerung von Pd‐Atomen in den Mesoporen eines graphitischen Kohlenstoffnitridpolymers. Die Analyse des Materials bestätigt die atomare Dispersion der Palladium‐Phase über die komplette Probe. Gegenüber nanopartikelbasierten Vergleichskatalysatoren zeigte sich die hohe Aktivität und Selektivität deutlich bei Anwendung in der kontinuierlichen Drei‐Phasen‐Hydrierung von Alkinen und Nitroarenen in einem Durchflussreaktor. Dichtefunktionalrechnungen ermöglichten die Erarbeitung fundamentaler Erkenntnisse betreffend Materialstruktur und erlaubten, die hohe katalytische Aktivität und Selektivität auf die einfache Wasserstoffaktivierung und Kohlenwasserstoffadsorption auf den atomar verteilten Pd‐Strukturen zurückzuführen.
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Citations
Cited by
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Single Pt Atoms Confined into a Metal–Organic Framework for Efficient Photocatalysis
Fang, X., Shang, Q., Wang, Y., Jiao, L., Yao, T., Li, Y., Zhang, Q., Luo, Y., & Jiang, H. (2018) · Advanced Materials · doi:10.1002/adma.201705112 · Cited by 837
An, S., Zhang, G., Wang, T., Zhang, W., Li, K., Song, C., Miller, J. T., Miao, S., Wang, J., & Guo, X. (2018) · ACS Nano · doi:10.1021/acsnano.8b04693 · Cited by 601
Zhang, L., Han, L., Liu, H., Liu, X., & Luo, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201706921 · Cited by 532
Strategies to break linear scaling relationships
Pérez-Ramírez, J., & López, N. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0376-6 · Cited by 528
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Metadata
- Authors
- Vilé, G., Albani, D., Nachtegaal, M., Chen, Z., Dontsova, D., Antonietti, M., López, N., & Pérez‐Ramírez, J.
- Venue
- Angewandte Chemie
- Publisher
- Wiley
- Published
- 2015-07-31
- Volume
- 127
- Issue
- 38
- Pages
- 11417-11422
- ISSN
- 0044-8249 (ISSN-L)
- 1521-3757
- OpenAlex
- W2149309416
- Cited by
- 506
- References
- 0
- FWCI
- 31.32
- Type
- journal article
- Language
- de
- Open access
- closed
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- Vilé, G., Albani, D., Nachtegaal, M., Chen, Z., Dontsova, D., Antonietti, M., López, N., & Pérez‐Ramírez, J. (2015). Ein stabiler “Single‐site”‐Palladiumkatalysator für Hydrierungen. Angewandte Chemie. https://doi.org/10.1002/ange.201505073
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