The DOI matches its Crossref record; 57 of the 57 references it cites were found in a registry or an index.
Single Pt Atoms Confined into a Metal–Organic Framework for Efficient Photocatalysis
Abstract
It is highly desirable yet remains challenging to improve the dispersion and usage of noble metal cocatalysts, beneficial to charge transfer in photocatalysis. Herein, for the first time, single Pt atoms are successfully confined into a metal–organic framework (MOF), in which electrons transfer from the MOF photosensitizer to the Pt acceptor for hydrogen production by water splitting under visible‐light irradiation. Remarkably, the single Pt atoms exhibit a superb activity, giving a turnover frequency of 35 h−1, ≈30 times that of Pt nanoparticles stabilized by the same MOF. Ultrafast transient absorption spectroscopy further unveils that the single Pt atoms confined into the MOF provide highly efficient electron transfer channels and density functional theory calculations indicate that the introduction of single Pt atoms into the MOF improves the hydrogen binding energy, thus greatly boosting the photocatalytic H 2 production activity.
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Cites
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Single-atom catalysis of CO oxidation using Pt1/FeOx
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Single-Atom Catalysts: A New Frontier in Heterogeneous Catalysis
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Metal–Organic Frameworks (MOFs)
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Cited by
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
Gao, C., Low, J., Long, R., Kong, T., Zhu, J., & Xiong, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00840 · Cited by 1,050
Metal–organic frameworks as a platform for clean energy applications
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Self-citationRecent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
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Metadata
- Authors
- Fang, X., Shang, Q., Wang, Y., Jiao, L., Yao, T., Li, Y., Zhang, Q., Luo, Y., & Jiang, H.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-01-08
- Volume
- 30
- Issue
- 7
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2782785851
- Cited by
- 837
- References
- 57
- FWCI
- 20.81
- Type
- journal article
- Language
- en
- Open access
- closed
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