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In Situ Generation of Highly Active Dissolved Palladium Species from Solid Catalysts—A Concept for the Activation of Aryl Chlorides in the Heck Reaction
Abstract
Needing a leach: Optimized palladium/metal oxide systems are highly active heterogeneous catalysts for the Heck reaction. Non-activated and deactivated aryl chlorides can be converted by palladium/zeolite (NaY) catalysts (see scheme). The dissolution of palladium (leaching) from the surface of the support, its redeposition, and the control of these equilibria are found to be crucial for the success of the reaction.
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Citations
Cited by
Nanoparticles as Recyclable Catalysts: The Frontier between Homogeneous and Heterogeneous Catalysis
Astruc, D., Lu, F., & Aranzaes, J. R. (2005) · Angewandte Chemie International Edition · doi:10.1002/anie.200500766 · Cited by 3,131
Carbon−Carbon Coupling Reactions Catalyzed by Heterogeneous Palladium Catalysts
Yin, & Liebscher, J. (2007) · Chemical Reviews · doi:10.1021/cr0505674 · Cited by 2,085
Phan, N. T. S., Van Der Sluys, M., & Jones, C. W. (2006) · Advanced Synthesis & Catalysis · doi:10.1002/adsc.200505473 · Cited by 1,905
de Vries, J. G. (2006) · Dalton Trans. · doi:10.1039/b506276b · Cited by 624
Alonso, F., Beletskaya, I. P., & Yus, M. (2005) · Tetrahedron · doi:10.1016/j.tet.2005.08.054 · Cited by 498
Metadata
- Authors
- Pröckl, S. S., Kleist, W., Gruber, M. A., & Köhler, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2004-03-24
- Volume
- 43
- Issue
- 14
- Pages
- 1881-1882
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2098045120
- Cited by
- 260
- References
- 0
- FWCI
- 16.52
- Type
- journal article
- Language
- en
- Open access
- closed
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- Pröckl, S. S., Kleist, W., Gruber, M. A., & Köhler, K. (2004). In Situ Generation of Highly Active Dissolved Palladium Species from Solid Catalysts—A Concept for the Activation of Aryl Chlorides in the Heck Reaction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200353473
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