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Alcohols as Electrophiles in CC Bond‐Forming Reactions: The Hydrogen Autotransfer Process
Abstract
The hydrogen autotransfer process involves an initial oxidative hydrogen elimination, followed by different types of reactions, and is completed with a reductive hydrogen addition to give the final product. The sequence allows the alkylation of different nucleophilic agents using environmentally benign alcohols as electrophiles, mild conditions, and soft bases, with water produced as the only waste material. Recent examples of modulating the organometallic catalyst have also lent themselves to expansion of the range of available substrates, as described in this Minireview.
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Cited by
Integration of chemical catalysis with extractive fermentation to produce fuels
Anbarasan, P., Baer, Z. C., Sreekumar, S., Gross, E., Binder, J. B., Blanch, H. W., Clark, D. S., & Toste, F. D. (2012) · Nature · doi:10.1038/nature11594 · Cited by 385
Recent approaches for C–C bond formation via direct dehydrative coupling strategies
Kumar, R., & Van der Eycken, E. V. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35397k · Cited by 294
Metadata
- Authors
- Guillena, G., Ramón, D. J., & Yus, M.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2007-03-16
- Volume
- 46
- Issue
- 14
- Pages
- 2358-2364
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2105905257
- Cited by
- 562
- References
- 0
- FWCI
- 20.20
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Alcohols as Electrophiles in CC Bond‐Forming Reactions: The Hydrogen Autotransfer Process. https://app.cochat.ai/papers/10.1002/anie.200603794
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- Guillena, G., Ramón, D. J., & Yus, M. (2007). Alcohols as Electrophiles in CC Bond‐Forming Reactions: The Hydrogen Autotransfer Process. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200603794
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