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Highly Efficient Catalyst Systems Using Iron Complexes with a Tetradentate PNNP Ligand for the Asymmetric Hydrogenation of Polar Bonds
Abstract
Iron competes with pricey ruthenium: The first catalyst systems using iron complexes for asymmetric H2 hydrogenation at 50 °C and asymmetric transfer hydrogenation at room temperature has been discovered. The transfer hydrogenation activity is similar to that of the best ruthenium catalyst. Surprisingly, the precatalysts have a tetradentate diiminodiphosphine ligand which has no NH functionality.
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Cited by
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Self-citationGunanathan, C., & Milstein, D. (2011) · Accounts of Chemical Research · doi:10.1021/ar2000265 · Cited by 1,078
Redox-active ligands in catalysis
Luca, O. R., & Crabtree, R. H. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35228a · Cited by 1,039
Efficient Hydrogenation of Ketones Catalyzed by an Iron Pincer Complex
Langer, R., Leitus, G., Ben‐David, Y., & Milstein, D. (2011) · Angewandte Chemie International Edition · doi:10.1002/anie.201007406 · Cited by 375
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Metadata
- Authors
- Sui‐Seng, C., Freutel, F., Lough, A. J., & Morris, R. H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2008-01-11
- Volume
- 47
- Issue
- 5
- Pages
- 940-943
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2108315037
- Cited by
- 354
- References
- 0
- FWCI
- 14.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sui‐Seng, C., Freutel, F., Lough, A. J., & Morris, R. H. (2008). Highly Efficient Catalyst Systems Using Iron Complexes with a Tetradentate PNNP Ligand for the Asymmetric Hydrogenation of Polar Bonds. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200705115
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