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Chiral Nanoscale Metal–Organic Tetrahedral Cages: Diastereoselective Self‐Assembly and Enantioselective Separation
Abstract
Cage rage: Chiral tetrahedral cages are diastereoselectively self-assembled from enantiopure C2-symmetric biphenyl bis(β-diketonate) linkers and C3-symmetric octahedral Fe3+ or Ga3+ ions (see picture; Fe purple, C blue, O red; cavity shown as an orange sphere). The porous polyhedra exhibit metal-dependent chiroptical behavior and act as hosts for the crystallization separation of racemic alcohols with up to 99.5 % ee.
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Citations
Cited by
Chiral metallosupramolecular architectures
Chen, L.-J., Yang, H.-B., & Shionoya, M. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00173h · Cited by 531
Metal–organic cages for molecular separations
Zhang, D., Ronson, T. K., Zou, Y.-Q., & Nitschke, J. R. (2021) · Nature Reviews Chemistry · doi:10.1038/s41570-020-00246-1 · Cited by 512
Separation of enantiomers by their enantiospecific interaction with achiral magnetic substrates
Banerjee-Ghosh, K., Ben Dor, O., Tassinari, F., Capua, E., Yochelis, S., Capua, A., Yang, S.-H., Parkin, S. S. P., Sarkar, S., Kronik, L., et al. (2018) · Science · doi:10.1126/science.aar4265 · Cited by 460
Pan, M., Wu, K., Zhang, J.-H., & Su, C.-Y. (2019) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.10.031 · Cited by 369
A Chiral Quadruple-Stranded Helicate Cage for Enantioselective Recognition and Separation
Xuan, W., Zhang, M., Liu, Y., Chen, Z., & Cui, Y. (2012) · Journal of the American Chemical Society · doi:10.1021/ja212132r · Cited by 349
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Metadata
- Authors
- Liu, T., Liu, Y., Xuan, W., & Cui, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2010-05-26
- Volume
- 49
- Issue
- 24
- Pages
- 4121-4124
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2101796159
- Cited by
- 202
- References
- 0
- FWCI
- 9.63
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, T., Liu, Y., Xuan, W., & Cui, Y. (2010). Chiral Nanoscale Metal–Organic Tetrahedral Cages: Diastereoselective Self‐Assembly and Enantioselective Separation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201000416
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