Cited by 365Enzyme Catalysis and ImmobilizationMetal-Catalyzed Oxygenation MechanismsAdvanced Nanomaterials in Catalysis

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Graphene‐Supported Hemin as a Highly Active Biomimetic Oxidation Catalyst

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Xue, Teng, Jiang, Shan, Qu, Yongquan, Su, Qiao, Cheng, Rui, Dubin, Sergey, Chiu, Chin‐Yi, Kaner, Richard, Huang, Yu, Duan, Xiangfeng·2012·Angewandte Chemie International Edition

DOI 10.1002/anie.201108400PMC PMC4249660

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Abstract

Well supported: stable hemin-graphene conjugates formed by immobilization of monomeric hemin on graphene, showed excellent catalytic activity, more than 10 times better than that of the recently developed hemin-hydrogel system and 100 times better than that of unsupported hemin. The catalysts also showed excellent binding affinities and catalytic efficiencies approaching that of natural enzymes.

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Authors: Xue, T., Jiang, S., Qu, Y., Su, Q., Cheng, R., Dubin, S., Chiu, C., Kaner, R., Huang, Y., & Duan, X.
Affiliations: University of California, Los Angeles (US)
California NanoSystems Institute (US)
Corresponding author: Huang, Yu
Duan, Xiangfeng
ORCID: Jiang, Shan
Qu, Yongquan
Cheng, Rui
Kaner, Richard
Huang, Yu
Duan, Xiangfeng
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2012-02-24
Volume: 51
Issue: 16
Pages: 3822-3825
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.201108400
PMC: PMC4249660
OpenAlex: W2144253455
Cited by: 365
References: 42
Citations by year: 2026: 6 · 2025: 13 · 2024: 8 · 2023: 12 · 2022: 19 · 2021: 29 · 2020: 30 · 2019: 29 · 2018: 40 · 2017: 38 · 2016: 29 · 2015: 30 · 2014: 34 · 2013: 38 · 2012: 10
FWCI: 14.31
Type: journal article
Language: en
Open access: bronze
doi.org
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
PubMed Central (acceptedVersion)
Funders: National Institutes of Health (1dp2od004342-01, 1dp2od007279-01)
Topics: Life Sciences › Biochemistry, Genetics and Molecular Biology › Molecular Biology › Enzyme Catalysis and Immobilization
Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Catalyzed Oxygenation Mechanisms
Physical Sciences › Materials Science › Materials Chemistry › Advanced Nanomaterials in Catalysis
Keywords: hemin, graphene, supported metalloporphyrins, enzyme mimics, catalytic efficiency, binding affinity
MeSH terms: Catalysis, Graphite, Hemin, Kinetics, Oxidation-Reduction, Oxides, Hydrogel, Polyethylene Glycol Dimethacrylate, Biomimetic Materials

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Graphene‐Supported Hemin as a Highly Active Biomimetic Oxidation Catalyst

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