The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Monolayer HNb3O8 for Selective Photocatalytic Oxidation of Benzylic Alcohols with Visible Light Response
Abstract
Monolayer HNb 3 O 8 2D nanosheets have been used as highly chemoselective and active photocatalysts for the selective oxidation of alcohols. The nanosheets exhibit improved photocatalytic activity over their layered counterparts. Results of in situ FTIR, DRS, ESR, and DFT calculations show the formation of surface complexes between the Lewis acid sites on HNb 3 O 8 2D nanosheets and alcohols. These complexes play a key role in the photocatalytic activity of the material. Furthermore, the unique structural features of the nanosheets contributed to their high photocatalytic activity. An electron transition from the coordinated alcohol species to surface Nb atoms takes place and initiates the aerobic oxidation of alcohols with high product selectivity under visible light irradiation. This reaction process is distinct from that of classic semiconductor photocatalysis.
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Cites
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
Wang, Q. H., Kalantar-Zadeh, K., Kis, A., Coleman, J. N., & Strano, M. S. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.193 · Cited by 16,374
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Progress, challenge and perspective of heterogeneous photocatalysts
Qu, Y., & Duan, X. (2013) · Chem. Soc. Rev. · doi:10.1039/c2cs35355e · Cited by 1,466
Cited by
Graphitic Carbon Nitride Polymers toward Sustainable Photoredox Catalysis
Zheng, Y., Lin, L., Wang, B., & Wang, X. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201501788 · Cited by 1,432
Qi, M.-Y., Li, Y.-H., Anpo, M., Tang, Z.-R., & Xu, Y.-J. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c04237 · Cited by 268
Xu, Y., Yin, X., Huang, Y., Du, P., & Zhang, B. (2015) · Chemistry – A European Journal · doi:10.1002/chem.201406642 · Cited by 63
Metadata
- Authors
- Liang, S., Wen, L., Lin, S., Bi, J., Feng, P., Fu, X., & Wu, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-02-12
- Volume
- 53
- Issue
- 11
- Pages
- 2951-2955
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2132512431
- Cited by
- 240
- References
- 3
- FWCI
- 6.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liang, S., Wen, L., Lin, S., Bi, J., Feng, P., Fu, X., & Wu, L. (2014). Monolayer HNb3O8 for Selective Photocatalytic Oxidation of Benzylic Alcohols with Visible Light Response. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201311280
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