The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Dynamic Diselenide Bonds: Exchange Reaction Induced by Visible Light without Catalysis
Abstract
Dynamic covalent bonds are extensively employed in dynamic combinatorial chemistry. The metathesis reaction of disulfide bonds is widely used, but requires catalysis or irradiation with ultraviolet (UV) light. It was found that diselenide bonds are dynamic covalent bonds and undergo dynamic exchange reactions under mild conditions for diselenide metathesis. This reaction is induced by irradiation with visible light and stops in the dark. The exchange is assumed to proceed through a radical mechanism, and experiments with 2,2,6,6‐tetramethylpiperidin‐1‐yloxyl (TEMPO) support this assumption. Furthermore, the reaction can be conducted in different solvents, including protic solvents. Diselenide metathesis can also be used to synthesize diselenide‐containing asymmetric block copolymers. This work thus entails the use of diselenide bonds as dynamic covalent bonds, the development of a dynamic exchange reaction under mild conditions, and an extension of selenium‐related dynamic chemistry.
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Dynamic Combinatorial Chemistry
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Cited by
Lai, Y., Kuang, X., Zhu, P., Huang, M., Dong, X., & Wang, D. (2018) · Advanced Materials · doi:10.1002/adma.201802556 · Cited by 686
Zhang, Z. P., Rong, M. Z., & Zhang, M. Q. (2018) · Progress in Polymer Science · doi:10.1016/j.progpolymsci.2018.03.002 · Cited by 586
Advances in redox-responsive drug delivery systems of tumor microenvironment
Guo, X., Cheng, Y., Zhao, X., Luo, Y., Chen, J., & Yuan, W.-E. (2018) · Journal of Nanobiotechnology · doi:10.1186/s12951-018-0398-2 · Cited by 459
Zhang, Q., Niu, S., Wang, L., Lopez, J., Chen, S., Cai, Y., Du, R., Liu, Y., Lai, J., Liu, L., et al. (2018) · Advanced Materials · doi:10.1002/adma.201801435 · Cited by 398
Li, Y., Li, W., Sun, A., Jing, M., Liu, X., Wei, L., Wu, K., & Fu, Q. (2021) · Materials Horizons · doi:10.1039/d0mh01447h · Cited by 316
Metadata
- Authors
- Ji, S., Cao, W., Yu, Y., & Xu, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-05-19
- Volume
- 53
- Issue
- 26
- Pages
- 6781-6785
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2118087633
- Cited by
- 337
- References
- 31
- FWCI
- 10.81
- Type
- journal article
- Language
- en
- Open access
- closed
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