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Harvesting Solar Light with Crystalline Carbon Nitrides for Efficient Photocatalytic Hydrogen Evolution
Abstract
Described herein is the photocatalytic hydrogen evolution using crystalline carbon nitrides (CNs) obtained by supramolecular aggregation followed by ionic melt polycondensation (IMP) using melamine and 2,4,6‐triaminopyrimidine as a dopant. The solid state NMR spectrum of 15 N‐enriched CN confirms the triazine as a building unit. Controlling the amount and arrangements of dopants in the CN structure can dramatically enhance the photocatalytic performance for H 2 evolution. The polytriazine imide (PTI) exhibits the apparent quantum efficiency (AQE) of 15 % at 400 nm. This method successfully enables a substantial amount of visible light to be harvested for H 2 evolution, and provides a promising route for the rational design of a variety of highly active crystalline CN photocatalysts.
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Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis
Yang, J., Wang, D., Han, H., & Li, C. (2013) · Accounts of Chemical Research · doi:10.1021/ar300227e · Cited by 2,848
Vrubel, H., Moehl, T., Grätzel, M., & Hu, X. (2013) · Chemical Communications · doi:10.1039/c3cc45416a · Cited by 335
Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Ye, C., Li, J.-X., Li, Z.-J., Li, X.-B., Fan, X.-B., Zhang, L.-P., Chen, B., Tung, C.-H., & Wu, L.-Z. (2015) · ACS Catalysis · doi:10.1021/acscatal.5b02185 · Cited by 490
Yi, S.-S., Yan, J.-M., Wulan, B.-R., Li, S.-J., Liu, K.-H., & Jiang, Q. (2017) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.07.046 · Cited by 420
Bai, Y., Wilbraham, L., Slater, B. J., Zwijnenburg, M. A., Sprick, R. S., & Cooper, A. I. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b03591 · Cited by 409
Zhang, G., Lan, Z.-A., & Wang, X. (2017) · Chemical Science · doi:10.1039/c7sc01747b · Cited by 357
Metadata
- Authors
- Bhunia, M. K., Yamauchi, K., & Takanabe, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-08-14
- Volume
- 53
- Issue
- 41
- Pages
- 11001-11005
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2129691811
- Cited by
- 345
- References
- 2
- FWCI
- 10.15
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bhunia, M. K., Yamauchi, K., & Takanabe, K. (2014). Harvesting Solar Light with Crystalline Carbon Nitrides for Efficient Photocatalytic Hydrogen Evolution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201405161
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