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Direct α‐Arylation of Ethers through the Combination of Photoredox‐Mediated CH Functionalization and the Minisci Reaction
Open accessAbstract
The direct α‐arylation of cyclic and acyclic ethers with heteroarenes has been accomplished through the design of a photoredox‐mediated CH functionalization pathway. Transiently generated α‐oxyalkyl radicals, produced from a variety of widely available ethers through hydrogen atom transfer (HAT), were coupled with a range of electron‐deficient heteroarenes in a Minisci‐type mechanism. This mild, visible‐light‐driven protocol allows direct access to medicinal pharmacophores of broad utility using feedstock substrates and a commercial photocatalyst.
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Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
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Photoredox-Catalyzed C–H Functionalization Reactions
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Taylor, A. P., Robinson, R. P., Fobian, Y. M., Blakemore, D. C., Jones, L. H., & Fadeyi, O. (2016) · Organic & Biomolecular Chemistry · doi:10.1039/c6ob00936k · Cited by 887
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Metadata
- Authors
- Jin, J., & MacMillan, D. W. C.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-12-02
- Volume
- 54
- Issue
- 5
- Pages
- 1565-1569
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2099395175
- Cited by
- 456
- References
- 1
- FWCI
- 16.33
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Jin, J., & MacMillan, D. W. C. (2015). Direct α‐Arylation of Ethers through the Combination of Photoredox‐Mediated CH Functionalization and the Minisci Reaction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201410432
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
