The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Conversion of Carbon Dioxide by Methane Reforming under Visible‐Light Irradiation: Surface‐Plasmon‐Mediated Nonpolar Molecule Activation
Abstract
A novel CO 2 photoreduction method, CO 2 conversion through methane reforming into syngas (DRM) was adopted as an efficient approach to not only reduce the environmental concentration of the greenhouse gas CO 2 but also realize the net energy storage from solar energy to chemical energy. For the first time it is reported that gold, which was generally regarded to be inactive in improving the performance of a catalyst in DRM under thermal conditions, enhanced the catalytic performance of Rh/SBA‐15 in DRM under visible‐light irradiation (1.7 times, CO 2 conversion increased from 2100 to 3600 μmol g−1 s−1). UV/Vis spectra and electromagnetic field simulation results revealed that the highly energetic electrons excited by local surface plasmon resonances of Au facilitated the polarization and activation of CO 2 and CH 4 with thermal assistance. This work provides a new route for CO 2 photoreduction and offers a distinctive method to photocatalytically activate nonpolar molecules.
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Citations
Cites
Recent advances in catalytic hydrogenation of carbon dioxide
Wang, W., Wang, S., Ma, X., & Gong, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15008a · Cited by 3,316
Cited by
Cocatalysts for Selective Photoreduction of CO2into Solar Fuels
Li, X., Yu, J., Jaroniec, M., & Chen, X. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00400 · Cited by 2,304
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Principles of photothermal gas-phase heterogeneous CO2 catalysis
Ghoussoub, M., Xia, M., Duchesne, P. N., Segal, D., & Ozin, G. (2019) · Energy & Environmental Science · doi:10.1039/c8ee02790k · Cited by 531
Solar-Energy-Mediated Methane Conversion
Song, H., Meng, X., Wang, Z.-J., Liu, H., & Ye, J. (2019) · Joule · doi:10.1016/j.joule.2019.06.023 · Cited by 478
Self-citationFrom Solar Energy to Fuels: Recent Advances in Light‐Driven C1 Chemistry
Chen, G., Waterhouse, G. I. N., Shi, R., Zhao, J., Li, Z., Wu, L., Tung, C., & Zhang, T. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201814313 · Cited by 396
Metadata
- Authors
- Liu, H., Meng, X., Dao, T. D., Zhang, H., Li, P., Chang, K., Wang, T., Li, M., Nagao, T., & Ye, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-08-13
- Volume
- 54
- Issue
- 39
- Pages
- 11545-11549
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2111447958
- Cited by
- 219
- References
- 1
- FWCI
- 3.52
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Liu, H., Meng, X., Dao, T. D., Zhang, H., Li, P., Chang, K., Wang, T., Li, M., Nagao, T., & Ye, J. (2015). Conversion of Carbon Dioxide by Methane Reforming under Visible‐Light Irradiation: Surface‐Plasmon‐Mediated Nonpolar Molecule Activation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201504933
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