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A Stable Single‐Site Palladium Catalyst for Hydrogenations
Open accessAbstract
We report the preparation and hydrogenation performance of a single‐site palladium catalyst that was obtained by the anchoring of Pd atoms into the cavities of mesoporous polymeric graphitic carbon nitride. The characterization of the material confirmed the atomic dispersion of the palladium phase throughout the sample. The catalyst was applied for three‐phase hydrogenations of alkynes and nitroarenes in a continuous‐flow reactor, showing its high activity and product selectivity in comparison with benchmark catalysts based on nanoparticles. Density functional theory calculations provided fundamental insights into the material structure and attributed the high catalyst activity and selectivity to the facile hydrogen activation and hydrocarbon adsorption on atomically dispersed Pd sites.
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Citations
Cited by
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Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Single Pt Atoms Confined into a Metal–Organic Framework for Efficient Photocatalysis
Fang, X., Shang, Q., Wang, Y., Jiao, L., Yao, T., Li, Y., Zhang, Q., Luo, Y., & Jiang, H. (2018) · Advanced Materials · doi:10.1002/adma.201705112 · Cited by 837
An, S., Zhang, G., Wang, T., Zhang, W., Li, K., Song, C., Miller, J. T., Miao, S., Wang, J., & Guo, X. (2018) · ACS Nano · doi:10.1021/acsnano.8b04693 · Cited by 601
Zhang, L., Han, L., Liu, H., Liu, X., & Luo, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201706921 · Cited by 532
Strategies to break linear scaling relationships
Pérez-Ramírez, J., & López, N. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0376-6 · Cited by 528
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Metadata
- Authors
- Vilé, G., Albani, D., Nachtegaal, M., Chen, Z., Dontsova, D., Antonietti, M., López, N., & Pérez‐Ramírez, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-07-31
- Volume
- 54
- Issue
- 38
- Pages
- 11265-11269
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2109694766
- Cited by
- 973
- References
- 0
- FWCI
- 36.26
- Type
- journal article
- Language
- en
- Open access
- green
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- Vilé, G., Albani, D., Nachtegaal, M., Chen, Z., Dontsova, D., Antonietti, M., López, N., & Pérez‐Ramírez, J. (2015). A Stable Single‐Site Palladium Catalyst for Hydrogenations. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201505073
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