The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Large‐Area, Free‐Standing, Two‐Dimensional Supramolecular Polymer Single‐Layer Sheets for Highly Efficient Electrocatalytic Hydrogen Evolution
Abstract
The rational construction of covalent or noncovalent organic two‐dimensional nanosheets is a fascinating target because of their promising applications in electronics, membrane technology, catalysis, sensing, and energy technologies. Herein, a large‐area (square millimeters) and free‐standing 2D supramolecular polymer (2DSP) single‐layer sheet (0.7–0.9 nm in thickness), comprising triphenylene‐fused nickel bis(dithiolene) complexes has been readily prepared by using the Langmuir–Blodgett method. Such 2DSPs exhibit excellent electrocatalytic activities for hydrogen generation from water with a Tafel slope of 80.5 mV decade−1 and an overpotential of 333 mV at 10 mA cm−2, which are superior to that of recently reported carbon nanotube supported molecular catalysts and heteroatom‐doped graphene catalysts. This work is promising for the development of novel free‐standing organic 2D materials for energy technologies.
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Cites
Electric Field Effect in Atomically Thin Carbon Films
Novoselov, K. S., Geim, A. K., Morozov, S. V., Jiang, D., Zhang, Y., Dubonos, S. V., Grigorieva, I. V., & Firsov, A. A. (2004) · Science · doi:10.1126/science.1102896 · Cited by 66,834
Kibsgaard, J., Chen, Z., Reinecke, B. N., & Jaramillo, T. F. (2012) · Nature Materials · doi:10.1038/nmat3439 · Cited by 3,234
Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
Voiry, D., Yamaguchi, H., Li, J., Silva, R., Alves, D. C. B., Fujita, T., Chen, M., Asefa, T., Shenoy, V. B., Eda, G., et al. (2013) · Nature Materials · doi:10.1038/nmat3700 · Cited by 2,641
Zou, X., Huang, X., Goswami, A., Silva, R., Sathe, B. R., Mikmeková, E., & Asefa, T. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201311111 · Cited by 979
Cited by
Electrochemical oxygen reduction catalysed by Ni3(hexaiminotriphenylene)2
Miner, E. M., Fukushima, T., Sheberla, D., Sun, L., Surendranath, Y., & Dincă, M. (2016) · Nature Communications · doi:10.1038/ncomms10942 · Cited by 710
Interface-Assisted Synthesis of 2D Materials: Trend and Challenges
Dong, R., Zhang, T., & Feng, X. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00056 · Cited by 710
Self-citationMitra, S., Sasmal, H. S., Kundu, T., Kandambeth, S., Illath, K., Díaz Díaz, D., & Banerjee, R. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b00925 · Cited by 587
Porous Polymers as Multifunctional Material Platforms toward Task‐Specific Applications
Wu, J., Xu, F., Li, S., Ma, P., Zhang, X., Liu, Q., Fu, R., & Wu, D. (2019) · Advanced Materials · doi:10.1002/adma.201802922 · Cited by 555
Recent progress in metal-organic frameworks as active materials for supercapacitors
Wang, K.-B., Xun, Q., & Zhang, Q. (2020) · EnergyChem · doi:10.1016/j.enchem.2019.100025 · Cited by 474
Metadata
- Authors
- Dong, R., Pfeffermann, M., Liang, H., Zheng, Z., Zhu, X., Zhang, J., & Feng, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-08-26
- Volume
- 54
- Issue
- 41
- Pages
- 12058-12063
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2137474022
- Cited by
- 621
- References
- 4
- FWCI
- 13.29
- Type
- journal article
- Language
- en
- Open access
- closed
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- Dong, R., Pfeffermann, M., Liang, H., Zheng, Z., Zhu, X., Zhang, J., & Feng, X. (2015). Large‐Area, Free‐Standing, Two‐Dimensional Supramolecular Polymer Single‐Layer Sheets for Highly Efficient Electrocatalytic Hydrogen Evolution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201506048
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