The DOI matches its Crossref record; 43 of the 43 references it cites were found in a registry or an index.
Electrochemical oxygen reduction catalysed by Ni3(hexaiminotriphenylene)2
Open accessAbstract
Control over the architectural and electronic properties of heterogeneous catalysts poses a major obstacle in the targeted design of active and stable non-platinum group metal electrocatalysts for the oxygen reduction reaction. Here we introduce Ni 3(HITP)2 (HITP=2, 3, 6, 7, 10, 11-hexaiminotriphenylene) as an intrinsically conductive metal-organic framework which functions as a well-defined, tunable oxygen reduction electrocatalyst in alkaline solution. Ni 3(HITP)2 exhibits oxygen reduction activity competitive with the most active non-platinum group metal electrocatalysts and stability during extended polarization. The square planar Ni-N 4 sites are structurally reminiscent of the highly active and widely studied non-platinum group metal electrocatalysts containing M-N 4 units. Ni 3(HITP)2 and analogues thereof combine the high crystallinity of metal-organic frameworks, the physical durability and electrical conductivity of graphitic materials, and the diverse yet well-controlled synthetic accessibility of molecular species. Such properties may enable the targeted synthesis and systematic optimization of oxygen reduction electrocatalysts as components of fuel cells and electrolysers for renewable energy applications.
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Cites
Covalent organic frameworks comprising cobalt porphyrins for catalytic CO 2 reduction in water
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Self-citationJahan, M., Liu, Z., & Loh, K. P. (2013) · Advanced Functional Materials · doi:10.1002/adfm.201300510 · Cited by 1,016
Electrocatalytically Active Graphene–Porphyrin MOF Composite for Oxygen Reduction Reaction
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Self-citationOn the Role of Metals in Nitrogen‐Doped Carbon Electrocatalysts for Oxygen Reduction
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Metadata
- Authors
- Miner, E. M., Fukushima, T., Sheberla, D., Sun, L., Surendranath, Y., & Dincă, M.
- Venue
- Nature Communications
- Published
- 2016-03-08
- Volume
- 7
- Issue
- 1
- Pages
- 10942-10942
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2312522982
- Cited by
- 710
- References
- 43
- FWCI
- 19.76
- Type
- journal article
- Language
- en
- Open access
- gold
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- Miner, E. M., Fukushima, T., Sheberla, D., Sun, L., Surendranath, Y., & Dincă, M. (2016). Electrochemical oxygen reduction catalysed by Ni3(hexaiminotriphenylene)2. Nature Communications. https://doi.org/10.1038/ncomms10942
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