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Dendrite‐Free Nanocrystalline Zinc Electrodeposition from an Ionic Liquid Containing Nickel Triflate for Rechargeable Zn‐Based Batteries
Abstract
Metallic zinc is a promising anode material for rechargeable Zn‐based batteries. However, the dendritic growth of zinc has prevented practical applications. Herein it is demonstrated that dendrite‐free zinc deposits with a nanocrystalline structure can be obtained by using nickel triflate as an additive in a zinc triflate containing ionic liquid. The formation of a thin layer of Zn–Ni alloy (η‐ and γ‐phases) on the surface and in the initial stages of deposition along with the formation of an interfacial layer on the electrode strongly affect the nucleation and growth of zinc. A well‐defined and uniform nanocrystalline zinc deposit with particle sizes of about 25 nm was obtained in the presence of Ni II. Further, it is shown that the nanocrystalline Zn exhibits a high cycling stability even after 50 deposition/stripping cycles. This strategy of introducing an inorganic metal salt in ionic liquid electrolytes can be considered as an efficient way to obtain dendrite‐free zinc.
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Citations
Cites
Application of ionic liquids to the electrodeposition of metals
Abbott, A. P., & McKenzie, K. J. (2006) · Physical Chemistry Chemical Physics · doi:10.1039/b607329h · Cited by 817
Cited by
A Metal-Organic Framework Host for Highly Reversible Dendrite-free Zinc Metal Anodes
Wang, Z., Huang, J., Guo, Z., Dong, X., Liu, Y., Wang, Y., & Xia, Y. (2019) · Joule · doi:10.1016/j.joule.2019.02.012 · Cited by 938
Xu, W., Zhao, K., Huo, W., Wang, Y., Yao, G., Gu, X., Cheng, H., Mai, L., Hu, C., & Wang, X. (2019) · Nano Energy · doi:10.1016/j.nanoen.2019.05.042 · Cited by 632
Alleviation of Dendrite Formation on Zinc Anodes via Electrolyte Additives
Guo, X., Zhang, Z., Li, J., Luo, N., Chai, G.-L., Miller, T. S., Lai, F., Shearing, P., Brett, D. J. L., Han, D., et al. (2021) · ACS Energy Letters · doi:10.1021/acsenergylett.0c02371 · Cited by 594
Inhibition of Zinc Dendrite Growth in Zinc‐Based Batteries
Lu, W., Xie, C., Zhang, H., & Li, X. (2018) · ChemSusChem · doi:10.1002/cssc.201801657 · Cited by 478
Advanced materials for zinc-based flow battery: development and challenge
Yuan, Z., Yin, Y., Xie, C., Zhang, H., Yao, Y., & Li, X. (2019) · Advanced Materials · doi:10.1002/adma.201902025 · Cited by 318
Metadata
- Authors
- Liu, Z., Cui, T., Pulletikurthi, G., Lahiri, A., Carstens, T., Olschewski, M., & Endres, F.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-01-28
- Volume
- 55
- Issue
- 8
- Pages
- 2889-2893
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2318100312
- Cited by
- 270
- References
- 1
- FWCI
- 9.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, Z., Cui, T., Pulletikurthi, G., Lahiri, A., Carstens, T., Olschewski, M., & Endres, F. (2016). Dendrite‐Free Nanocrystalline Zinc Electrodeposition from an Ionic Liquid Containing Nickel Triflate for Rechargeable Zn‐Based Batteries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201509364
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