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Nitrogen, Phosphorus, and Sulfur Co‐Doped Hollow Carbon Shell as Superior Metal‐Free Catalyst for Selective Oxidation of Aromatic Alkanes
Open accessAbstract
Metal‐free heteroatom‐doped carbocatalysts with a high surface area are desirable for catalytic reactions. In this study, we found an efficient strategy to prepare nitrogen, phosphorus, and sulfur co‐doped hollow carbon shells (denote as NPS‐HCS) with a surface area of 1020 m 2 g−1. Using a poly(cyclotriphosphazene‐co‐4,4′‐sulfonyldiphenol) (PZS) shell as carbon source and N, P, S‐doping source, and the ZIF‐67 core as structural template as well as extra N‐doping source, NPS‐HCS were obtained with a high surface area and superhydrophilicity. All these features render the prepared NPS‐HCS a superior metal‐free carbocatalyst for the selective oxidation of aromatic alkanes in aqueous solution. This study provides a reliable and facile route to prepare doped carbocatalysts with enhanced catalytic properties.
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Zhang, J., Qu, L., Shi, G., Liu, J., Chen, J., & Dai, L. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201510495 · Cited by 873
Cited by
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Gao, K., Wang, B., Tao, L., Cunning, B. V., Zhang, Z., Wang, S., Ruoff, R. S., & Qu, L. (2019) · Advanced Materials · doi:10.1002/adma.201805121 · Cited by 486
Yang, H., Bradley, S. J., Chan, A., Waterhouse, G. I. N., Nann, T., Kruger, P. E., & Telfer, S. G. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b06736 · Cited by 284
Controllable Syntheses of MOF‐Derived Materials
Zou, K., & Li, Z. (2018) · Chemistry – A European Journal · doi:10.1002/chem.201705415 · Cited by 172
Metadata
- Authors
- Yang, S., Peng, L., Huang, P., Wang, X., Sun, Y., Cao, C., & Song, W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-02-17
- Volume
- 55
- Issue
- 12
- Pages
- 4016-4020
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2283588039
- Cited by
- 295
- References
- 1
- FWCI
- 20.94
- Type
- journal article
- Language
- en
- Open access
- green
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- Yang, S., Peng, L., Huang, P., Wang, X., Sun, Y., Cao, C., & Song, W. (2016). Nitrogen, Phosphorus, and Sulfur Co‐Doped Hollow Carbon Shell as Superior Metal‐Free Catalyst for Selective Oxidation of Aromatic Alkanes. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201600455
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