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Aggregation‐Induced Delayed Fluorescence Based on Donor/Acceptor‐Tethered Janus Carborane Triads: Unique Photophysical Properties of Nondoped OLEDs
Abstract
Luminescent materials consisting of boron clusters, such as carboranes, have attracted immense interest in recent years. In this study, luminescent organic–inorganic conjugated systems based on o‐carboranes directly bonded to electron‐donating and electron‐accepting π‐conjugated units were elaborated as novel optoelectronic materials. These o‐carborane derivatives simultaneously possessed aggregation‐induced emission (AIE) and thermally activated delayed fluorescence (TADF) capabilities, and showed strong yellow‐to‐red emissions with high photoluminescence quantum efficiencies of up to 97 % in their aggregated states or in solid neat films. Organic light‐emitting diodes utilizing these o‐carborane derivatives as a nondoped emission layer exhibited maximum external electroluminescence quantum efficiencies as high as 11 %, originating from TADF.
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Cites
Aggregation-induced emission of 1-methyl-1,2,3,4,5-pentaphenylsilole
Luo, J., Xie, Z., Lam, J. W. Y., Cheng, L., Tang, B. Z., Chen, H., Qiu, C., Kwok, H. S., Zhan, X., Liu, Y., et al. (2001) · Chemical Communications · doi:10.1039/b105159h · Cited by 8,358
An, B.-K., Gierschner, J., & Park, S. Y. (2012) · Accounts of Chemical Research · doi:10.1021/ar2001952 · Cited by 743
Cited by
Recent advances in organic thermally activated delayed fluorescence materials
Yang, Z., Mao, Z., Xie, Z., Zhang, Y., Liu, S., Zhao, J., Xu, J., Chi, Z., & Aldred, M. P. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00368k · Cited by 2,395
All-organic thermally activated delayed fluorescence materials for organic light-emitting diodes
Liu, Y., Li, C., Ren, Z., Yan, S., & Bryce, M. R. (2018) · Nature Reviews Materials · doi:10.1038/natrevmats.2018.20 · Cited by 1,644
Aggregation-induced emission: fundamental understanding and future developments
Chen, Y., Lam, J. W. Y., Kwok, R. T. K., Liu, B., & Tang, B. Z. (2019) · Materials Horizons · doi:10.1039/c8mh01331d · Cited by 891
Photosensitizers with Aggregation‐Induced Emission: Materials and Biomedical Applications
Hu, F., Xu, S., & Liu, B. (2018) · Advanced Materials · doi:10.1002/adma.201801350 · Cited by 859
Aggregate Science: From Structures to Properties
Zhang, H., Zhao, Z., Turley, A. T., Wang, L., McGonigal, P. R., Tu, Y., Li, Y., Wang, Z., Kwok, R. T. K., Lam, J. W. Y., et al. (2020) · Advanced Materials · doi:10.1002/adma.202001457 · Cited by 518
Metadata
- Authors
- Furue, R., Nishimoto, T., Park, I. S., Lee, J., & Yasuda, T.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-05-04
- Volume
- 55
- Issue
- 25
- Pages
- 7171-7175
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2347133646
- Cited by
- 464
- References
- 2
- FWCI
- 26.63
- Type
- journal article
- Language
- en
- Open access
- closed
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- Furue, R., Nishimoto, T., Park, I. S., Lee, J., & Yasuda, T. (2016). Aggregation‐Induced Delayed Fluorescence Based on Donor/Acceptor‐Tethered Janus Carborane Triads: Unique Photophysical Properties of Nondoped OLEDs. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201603232
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