The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Molecular Engineering of Conjugated Polybenzothiadiazoles for Enhanced Hydrogen Production by Photosynthesis
Abstract
The search for metal‐free organic photocatalysts for H 2 production from water using visible light remains a key challenge. Reported herein is a molecular structural design of pure organic photocatalysts, derived from conjugated polybenzothiadiazoles, for photocatalytic H 2 evolution using visible light. By alternating the substitution position of the electron‐withdrawing benzothiadizole unit on the phenyl unit as a comonomer, various polymers with either one‐ or three‐dimensional structures were synthesized and the effect of the molecular structure on their catalytic activity was investigated. Photocatalytic H 2 evolution efficiencies up to 116 μmol h−1 were observed by employing the linear polymer based on a phenyl‐benzothiadiazole alternating main chain, with an apparent quantum yield (AQY) of 4.01 % at 420 nm using triethanolamine as the sacrificial agent.
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Citations
Cites
Photocatalytic Water Splitting: Recent Progress and Future Challenges
Maeda, K., & Domen, K. (2010) · The Journal of Physical Chemistry Letters · doi:10.1021/jz1007966 · Cited by 2,739
Wang, Q., Hisatomi, T., Jia, Q., Tokudome, H., Zhong, M., Wang, C., Pan, Z., Takata, T., Nakabayashi, M., Shibata, N., et al. (2016) · Nature Materials · doi:10.1038/nmat4589 · Cited by 1,684
Cited by
Sulfone-containing covalent organic frameworks for photocatalytic hydrogen evolution from water
Wang, X., Chen, L., Chong, S. Y., Little, M. A., Wu, Y., Zhu, W.-H., Clowes, R., Yan, Y., Zwijnenburg, M. A., Sprick, R. S., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0141-5 · Cited by 1,320
Self-citationCheng, C., He, B., Fan, J., Cheng, B., Cao, S., & Yu, J. (2021) · Advanced Materials · doi:10.1002/adma.202100317 · Cited by 888
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Bi, S., Yang, C., Zhang, W., Xu, J., Liu, L., Wu, D., Wang, X., Han, Y., Liang, Q., & Zhang, F. (2019) · Nature Communications · doi:10.1038/s41467-019-10504-6 · Cited by 616
Self-citationPorous Polymers as Multifunctional Material Platforms toward Task‐Specific Applications
Wu, J., Xu, F., Li, S., Ma, P., Zhang, X., Liu, Q., Fu, R., & Wu, D. (2019) · Advanced Materials · doi:10.1002/adma.201802922 · Cited by 555
Metadata
- Authors
- Yang, C., Ma, B. C., Zhang, L., Lin, S., Ghasimi, S., Landfester, K., Zhang, K. A. I., & Wang, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-06-15
- Volume
- 55
- Issue
- 32
- Pages
- 9202-9206
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2442970291
- Cited by
- 390
- References
- 2
- FWCI
- 13.59
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, C., Ma, B. C., Zhang, L., Lin, S., Ghasimi, S., Landfester, K., Zhang, K. A. I., & Wang, X. (2016). Molecular Engineering of Conjugated Polybenzothiadiazoles for Enhanced Hydrogen Production by Photosynthesis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201603532
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