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Amorphous Li2O2: Chemical Synthesis and Electrochemical Properties
Abstract
When aprotic Li–O 2 batteries discharge, the product phase formed in the cathode often contains two different morphologies, that is, crystalline and amorphous Li 2 O 2. The morphology of Li 2 O 2 impacts strongly on the electrochemical performance of Li–O 2 cells in terms of energy efficiency and rate capability. Crystalline Li 2 O 2 is readily available and its properties have been studied in depth for Li–O 2 batteries. However, little is known about the amorphous Li 2 O 2 because of its rarity in high purity. Herein, amorphous Li 2 O 2 has been synthesized by a rapid reaction of tetramethylammonium superoxide and LiClO 4 in solution, and its amorphous nature has been confirmed by a range of techniques. Compared with its crystalline siblings, amorphous Li 2 O 2 demonstrates enhanced charge‐transport properties and increased electro‐oxidation kinetics, manifesting itself a desirable discharge phase for high‐performance Li–O 2 batteries.
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Ostwald processes and mineral paragenesis in sediments
Morse, J. W., & Casey, W. H. (1988) · American Journal of Science · doi:10.2475/ajs.288.6.537 · Cited by 310
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Rational Design of MXene/1T‐2H MoS2‐C Nanohybrids for High‐Performance Lithium–Sulfur Batteries
Zhang, Y., Mu, Z., Yang, C., Xu, Z., Zhang, S., Zhang, X., Li, Y., Lai, J., Sun, Z., Yang, Y., et al. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201707578 · Cited by 417
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Recent advances in understanding Li–CO2 electrochemistry
Liu, B., Sun, Y., Liu, L., Chen, J., Yang, B., Xu, S., & Yan, X. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03417f · Cited by 317
Interstitial Hydrogen Atom Modulation to Boost Hydrogen Evolution in Pd-Based Alloy Nanoparticles
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Metadata
- Authors
- Zhang, Y., Cui, Q., Zhang, X., McKee, W. C., Xu, Y., Ling, S., Li, H., Zhong, G., Yang, Y., & Peng, Z.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-08-03
- Volume
- 55
- Issue
- 36
- Pages
- 10717-10721
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3215852057
- Cited by
- 161
- References
- 1
- FWCI
- 11.13
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, Y., Cui, Q., Zhang, X., McKee, W. C., Xu, Y., Ling, S., Li, H., Zhong, G., Yang, Y., & Peng, Z. (2016). Amorphous Li2O2: Chemical Synthesis and Electrochemical Properties. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201605228
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