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A Modulator‐Induced Defect‐Formation Strategy to Hierarchically Porous Metal–Organic Frameworks with High Stability
Abstract
The pore size enlargement and structural stability have been recognized as two crucial targets, which are rarely achieved together, in the development of metal–organic frameworks (MOFs). Herein, we have developed a versatile modulator‐induced defect‐formation strategy, in the presence of monocarboxylic acid as a modulator and an insufficient amount of organic ligand, successfully realizing the controllable synthesis of hierarchically porous MOFs (HP‐MOFs) with high stability and tailorable pore characters. Remarkably, the integration of high stability and large mesoporous property enables these HP‐MOFs to be important porous platforms for applications involving large molecules, especially in catalysis.
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Cited by
Ordered macro-microporous metal-organic framework single crystals
Shen, K., Zhang, L., Chen, X., Liu, L., Zhang, D., Han, Y., Chen, J., Long, J., Luque, R., Li, Y., et al. (2018) · Science · doi:10.1126/science.aao3403 · Cited by 1,207
Pristine Metal–Organic Frameworks and their Composites for Energy Storage and Conversion
Liang, Z., Qu, C., Guo, W., Zou, R., & Xu, Q. (2018) · Advanced Materials · doi:10.1002/adma.201702891 · Cited by 787
Feng, L., Yuan, S., Zhang, L.-L., Tan, K., Li, J.-L., Kirchon, A., Liu, L.-M., Zhang, P., Han, Y., Chabal, Y. J., et al. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.7b12916 · Cited by 423
Pullen, S., & Clever, G. H. (2018) · Accounts of Chemical Research · doi:10.1021/acs.accounts.8b00415 · Cited by 363
Xiang, W., Zhang, Y., Chen, Y., Liu, C.-J., & Tu, X. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta08009h · Cited by 359
Metadata
- Authors
- Cai, G., & Jiang, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-12-08
- Volume
- 56
- Issue
- 2
- Pages
- 563-567
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2560238774
- Cited by
- 663
- References
- 0
- FWCI
- 20.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cai, G., & Jiang, H. (2017). A Modulator‐Induced Defect‐Formation Strategy to Hierarchically Porous Metal–Organic Frameworks with High Stability. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201610914
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