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Microtubular Self‐Assembly of Covalent Organic Frameworks
Open accessAbstract
Despite significant progress in the synthesis of covalent organic frameworks (COFs), reports on the precise construction of template‐free nano‐ and microstructures of such materials have been rare. In the quest for dye‐containing porous materials, a novel conjugated framework DPP‐TAPP‐COF with an enhanced absorption capability up to λ=800 nm has been synthesized by utilizing reversible imine condensations between 5,10,15,20‐tetrakis(4‐aminophenyl)porphyrin (TAPP) and a diketopyrrolopyrrole (DPP) dialdehyde derivative. Surprisingly, the obtained COF exhibited spontaneous aggregation into hollow microtubular assemblies with outer and inner tube diameters of around 300 and 90 nm, respectively. A detailed mechanistic investigation revealed the time‐dependent transformation of initial sheet‐like agglomerates into the tubular microstructures.
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Gower, L. B. (2008) · Chemical Reviews · doi:10.1021/cr800443h · Cited by 1,086
Cited by
Covalent Organic Framework Photocatalysts: Structures and Applications
Wang, H., Wang, H., Wang, Z., Tang, L., Zeng, G., Xu, P., Chen, M., Xiong, T., Zhou, C., Li, X., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00278j · Cited by 1,301
Chen, R., Shi, J., Ma, Y., Lin, G., Lang, X., & Wang, C. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201902543 · Cited by 697
Opportunities of Covalent Organic Frameworks for Advanced Applications
Song, Y., Sun, Q., Aguila, B., & Ma, S. (2019) · Advanced Science · doi:10.1002/advs.201801410 · Cited by 586
Recent advances of multi-dimensional porphyrin-based functional materials in photodynamic therapy
Tian, J., Huang, B., Nawaz, M. H., & Zhang, W. (2020) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2020.213410 · Cited by 369
Landscaping Covalent Organic Framework Nanomorphologies
Sasmal, H. S., Kumar Mahato, A., Majumder, P., & Banerjee, R. (2022) · Journal of the American Chemical Society · doi:10.1021/jacs.2c02301 · Cited by 299
Metadata
- Authors
- Gole, B., Stepanenko, V., Rager, S., Grüne, M., Medina, D. D., Bein, T., Würthner, F., & Beuerle, F.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-12-13
- Volume
- 57
- Issue
- 3
- Pages
- 846-850
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2766160225
- Cited by
- 216
- References
- 1
- FWCI
- 7.57
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Gole, B., Stepanenko, V., Rager, S., Grüne, M., Medina, D. D., Bein, T., Würthner, F., & Beuerle, F. (2018). Microtubular Self‐Assembly of Covalent Organic Frameworks. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201708526
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