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A 3D Nanostructured Hydrogel‐Framework‐Derived High‐Performance Composite Polymer Lithium‐Ion Electrolyte
Abstract
Solid‐state electrolytes have emerged as a promising alternative to existing liquid electrolytes for next generation Li‐ion batteries for better safety and stability. Of various types of solid electrolytes, composite polymer electrolytes exhibit acceptable Li‐ion conductivity due to the interaction between nanofillers and polymer. Nevertheless, the agglomeration of nanofillers at high concentration has been a major obstacle for improving Li‐ion conductivity. In this study, we designed a three‐dimensional (3D) nanostructured hydrogel‐derived Li 0.35 La 0.55 TiO 3 (LLTO) framework, which was used as a 3D nanofiller for high‐performance composite polymer Li‐ion electrolyte. The systematic percolation study revealed that the pre‐percolating structure of LLTO framework improved Li‐ion conductivity to 8.8×10−5 S cm−1 at room temperature.
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Cited by
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Ionic Conduction in Polymer‐Based Solid Electrolytes
Li, Z., Fu, J., Zhou, X., Gui, S., Wei, L., Yang, H., Li, H., & Guo, X. (2023) · Advanced Science · doi:10.1002/advs.202201718 · Cited by 678
Self-citationMussel-inspired hydrogels: From design principles to promising applications
Zhang, C., Wu, B., Zhou, Y., Zhou, F., Liu, W., & Wang, Z. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00849g · Cited by 653
Yang, H., & Wu, N. (2022) · Energy Science & Engineering · doi:10.1002/ese3.1163 · Cited by 586
Recent progress on solid-state hybrid electrolytes for solid-state lithium batteries
Liang, J., Luo, J., Sun, Q., Yang, X., Li, R., & Sun, X. (2019) · Energy Storage Materials · doi:10.1016/j.ensm.2019.06.021 · Cited by 365
Metadata
- Authors
- Bae, J., Li, Y., Zhang, J., Zhou, X., Zhao, F., Shi, Y., Goodenough, J. B., & Yu, G.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-01-16
- Volume
- 57
- Issue
- 8
- Pages
- 2096-2100
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2782457318
- Cited by
- 656
- References
- 0
- FWCI
- 27.19
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bae, J., Li, Y., Zhang, J., Zhou, X., Zhao, F., Shi, Y., Goodenough, J. B., & Yu, G. (2018). A 3D Nanostructured Hydrogel‐Framework‐Derived High‐Performance Composite Polymer Lithium‐Ion Electrolyte. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201710841
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