The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
Regulation of Coordination Number over Single Co Sites: Triggering the Efficient Electroreduction of CO2
Abstract
The design of active, selective, and stable CO 2 reduction electrocatalysts is still challenging. A series of atomically dispersed Co catalysts with different nitrogen coordination numbers were prepared and their CO 2 electroreduction catalytic performance was explored. The best catalyst, atomically dispersed Co with two‐coordinate nitrogen atoms, achieves both high selectivity and superior activity with 94 % CO formation Faradaic efficiency and a current density of 18.1 mA cm−2 at an overpotential of 520 mV. The CO formation turnover frequency reaches a record value of 18 200 h−1, surpassing most reported metal‐based catalysts under comparable conditions. Our experimental and theoretical results demonstrate that lower a coordination number facilitates activation of CO 2 to the CO 2.− intermediate and hence enhances CO 2 electroreduction activity.
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Cites
Enhanced electrocatalytic CO2 reduction via field-induced reagent concentration
Liu, M., Pang, Y., Zhang, B., De Luna, P., Voznyy, O., Xu, J., Zheng, X., Dinh, C. T., Fan, F., Cao, C., et al. (2016) · Nature · doi:10.1038/nature19060 · Cited by 2,000
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Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Self-citationElectroreduction of carbon monoxide to liquid fuel on oxide-derived nanocrystalline copper
Li, C. W., Ciston, J., & Kanan, M. W. (2014) · Nature · doi:10.1038/nature13249 · Cited by 1,728
Recent Advances in Inorganic Heterogeneous Electrocatalysts for Reduction of Carbon Dioxide
Zhu, D. D., Liu, J. L., & Qiao, S. Z. (2016) · Advanced Materials · doi:10.1002/adma.201504766 · Cited by 1,594
Ionic Liquid–Mediated Selective Conversion of CO 2 to CO at Low Overpotentials
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Tuning the MoS 2 Edge-Site Activity for Hydrogen Evolution via Support Interactions
Tsai, C., Abild-Pedersen, F., & Nørskov, J. K. (2014) · Nano Letters · doi:10.1021/nl404444k · Cited by 760
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Designing materials for electrochemical carbon dioxide recycling
Ross, M. B., De Luna, P., Li, Y., Dinh, C.-T., Kim, D., Yang, P., & Sargent, E. H. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0306-7 · Cited by 1,302
Self-citationSingle atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Pu, Z., Liu, T., Amiinu, I. S., Cheng, R., Wang, P., Zhang, C., Ji, P., Hu, W., Liu, J., & Mu, S. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202004009 · Cited by 604
Yin, X., Wang, H., Tang, S., Lu, X., Shu, M., Si, R., & Lu, T. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201804817 · Cited by 594
Defect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
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Metadata
- Authors
- Wang, X., Chen, Z., Zhao, X., Yao, T., Chen, W., You, R., Zhao, C., Wu, G., Wang, J., Huang, W., Yang, J., Hong, X., Wei, S., Wu, Y., & Li, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-01-16
- Volume
- 57
- Issue
- 7
- Pages
- 1944-1948
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2779952271
- Cited by
- 1,120
- References
- 7
- FWCI
- 25.62
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, X., Chen, Z., Zhao, X., Yao, T., Chen, W., You, R., Zhao, C., Wu, G., Wang, J., Huang, W., Yang, J., Hong, X., Wei, S., Wu, Y., & Li, Y. (2018). Regulation of Coordination Number over Single Co Sites: Triggering the Efficient Electroreduction of CO2. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201712451
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