The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Photocatalytic Hydrogen Production Coupled with Selective Benzylamine Oxidation over MOF Composites
Abstract
Photocatalytic water splitting requires separation of the mixed H 2 and O 2 products and is often hampered by the sluggish O 2‐producing half reaction. An approach is now reported to address these issues by coupling the H 2‐producing half reaction with value‐added benzylamine oxidation reaction using metal–organic framework (MOF) composites. Upon MOF photoexcitation, the electrons rapidly reduce the protons to generate H 2 and the holes promote considerable benzylamine oxidation to N‐benzylbenzaldimine with high selectivity. Further experimental characterizations and theoretical calculation reveal that the highly conjugated s‐triazine strut in the MOF structure is crucial to the efficient charge separation and excellent photocatalytic activity.
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Citations
Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
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Cited by
Kampouri, S., & Stylianou, K. C. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b00332 · Cited by 298
Xu, M., Li, D., Sun, K., Jiao, L., Xie, C., Ding, C., & Jiang, H. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202104219 · Cited by 280
Self-citationZhang, F., Feng, L., Jia, C., Wu, Y., Liu, J., Shuai, X., & Cao, Z. (2023) · Nano Today · doi:10.1016/j.nantod.2022.101708 · Cited by 26
Metadata
- Authors
- Liu, H., Xu, C., Li, D., & Jiang, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-03-30
- Volume
- 57
- Issue
- 19
- Pages
- 5379-5383
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2791958841
- Cited by
- 542
- References
- 4
- FWCI
- 13.35
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, H., Xu, C., Li, D., & Jiang, H. (2018). Photocatalytic Hydrogen Production Coupled with Selective Benzylamine Oxidation over MOF Composites. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201800320
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