The DOI matches its Crossref record; 50 of the 50 references it cites were found in a registry or an index.
Interfacial Microenvironment Modulation Boosting Electron Transfer between Metal Nanoparticles and MOFs for Enhanced Photocatalysis
Abstract
Interfacial electron transfer between cocatalyst and photosensitizer is key in heterogeneous photocatalysis, yet the underlying mechanism remains subtle and unclear. Surfactant coated on the metal cocatalysts, greatly modulating the microenvironment of catalytic sites, is largely ignored. Herein, a series of Pt co‐catalysts with modulated microenvironments, including polyvinylpyrrolidone (PVP) capped Pt nanoparticles (denoted as Pt PVP), Pt with partially removed PVP (Pt rPVP), and clean Pt without PVP (Pt), were encapsulated into a metal–organic framework (MOF), UiO‐66‐NH 2, to afford Pt PVP@UiO‐66‐NH 2, Pt rPVP@UiO‐66‐NH 2, and Pt@UiO‐66‐NH 2, respectively, for photocatalytic hydrogen production. The PVP appears to have a negative influence on the interfacial electron transfer between Pt and the MOF. Compared with Pt PVP@UiO‐66‐NH 2, the removal of interfacial PVP improves the sluggish kinetics of electron transfer, boosting photocatalytic hydrogen production.
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Cites
The Chemistry and Applications of Metal-Organic Frameworks
Furukawa, H., Cordova, K. E., O’Keeffe, M., & Yaghi, O. M. (2013) · Science · doi:10.1126/science.1230444 · Cited by 16,945
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Metal–Organic Frameworks (MOFs)
Zhou, H.-C. “., & Kitagawa, S. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs90059f · Cited by 4,125
Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis
Yang, J., Wang, D., Han, H., & Li, C. (2013) · Accounts of Chemical Research · doi:10.1021/ar300227e · Cited by 2,848
Wang, Q., & Domen, K. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00201 · Cited by 2,809
Earth-abundant cocatalysts for semiconductor-based photocatalytic water splitting
Ran, J., Zhang, J., Yu, J., Jaroniec, M., & Qiao, S. Z. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60425j · Cited by 2,529
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Metal–organic frameworks meet metal nanoparticles: synergistic effect for enhanced catalysis
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Self-citationFu, Y., Sun, D., Chen, Y., Huang, R., Ding, Z., Fu, X., & Li, Z. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201108357 · Cited by 1,741
Metadata
- Authors
- Xu, M., Li, D., Sun, K., Jiao, L., Xie, C., Ding, C., & Jiang, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2021-06-24
- Volume
- 60
- Issue
- 30
- Pages
- 16372-16376
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3160146677
- Cited by
- 280
- References
- 50
- FWCI
- 9.15
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xu, M., Li, D., Sun, K., Jiao, L., Xie, C., Ding, C., & Jiang, H. (2021). Interfacial Microenvironment Modulation Boosting Electron Transfer between Metal Nanoparticles and MOFs for Enhanced Photocatalysis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202104219
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