The DOI matches its Crossref record; 45 of the 45 references it cites were found in a registry or an index.
Electrochemical Exfoliation of Pillared‐Layer Metal–Organic Framework to Boost the Oxygen Evolution Reaction
Abstract
Two‐dimensional (2D) materials and ultrathin nanosheets are advantageous for elevating the catalysis performance and elucidating the catalysis mechanism of heterogeneous catalysts, but they are mostly restricted to inorganic or organic materials based on covalent bonds. We report an electrochemical/chemical exfoliation strategy for synthesizing metal–organic 2D materials based on coordination bonds. A catechol functionalized ligand is used as the redox active pillar to construct a pillared‐layer framework. When the 3D pillared‐layer MOF serves as an electrocatalyst for water oxidation (pH 13), the pillar ligands can be oxidized in situ and removed. The remaining ultrathin (2 nm) nanosheets of the metal–organic layers are an efficient catalyst with overpotentials as low as 211 mV at 10 mA cm−2 and a turnover frequency as high as 30 s−1 at an overpotential of 300 mV.
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Cites
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Recent Advances in Ultrathin Two-Dimensional Nanomaterials
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In Situ Formation of an Oxygen-Evolving Catalyst in Neutral Water Containing Phosphate and Co 2+
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Self-citationUltrathin metal–organic framework nanosheets for electrocatalytic oxygen evolution
Zhao, S., Wang, Y., Dong, J., He, C.-T., Yin, H., An, P., Zhao, K., Zhang, X., Gao, C., Zhang, L., et al. (2016) · Nature Energy · doi:10.1038/nenergy.2016.184 · Cited by 2,602
Self-citationConductive MOF electrodes for stable supercapacitors with high areal capacitance
Sheberla, D., Bachman, J. C., Elias, J. S., Sun, C.-J., Shao-Horn, Y., & Dincă, M. (2017) · Nature Materials · doi:10.1038/nmat4766 · Cited by 2,370
Postsynthetic Methods for the Functionalization of Metal–Organic Frameworks
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Catalysis with two-dimensional materials and their heterostructures
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A highly active and stable IrO x /SrIrO 3 catalyst for the oxygen evolution reaction
Seitz, L. C., Dickens, C. F., Nishio, K., Hikita, Y., Montoya, J., Doyle, A., Kirk, C., Vojvodic, A., Hwang, H. Y., Norskov, J. K., et al. (2016) · Science · doi:10.1126/science.aaf5050 · Cited by 2,196
Cited by
Xu, H., Fei, B., Cai, G., Ha, Y., Liu, J., Jia, H., Zhang, J., Liu, M., & Wu, R. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902714 · Cited by 332
Self-citationXu, C., Zhang, M., Yin, X., Gao, Q., Jiang, S., Cheng, J., Kong, X., Liu, B., & Peng, H.-Q. (2023) · Journal of Materials Chemistry A · doi:10.1039/d3ta02293e · Cited by 65
Metadata
- Authors
- Huang, J., Li, Y., Huang, R., He, C., Gong, L., Hu, Q., Wang, L., Xu, Y., Tian, X., Liu, S., Ye, Z., Wang, F., Zhou, D., Zhang, W., & Zhang, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-03-13
- Volume
- 57
- Issue
- 17
- Pages
- 4632-4636
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2793258248
- Cited by
- 341
- References
- 45
- FWCI
- 10.52
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, J., Li, Y., Huang, R., He, C., Gong, L., Hu, Q., Wang, L., Xu, Y., Tian, X., Liu, S., Ye, Z., Wang, F., Zhou, D., Zhang, W., & Zhang, J. (2018). Electrochemical Exfoliation of Pillared‐Layer Metal–Organic Framework to Boost the Oxygen Evolution Reaction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201801029
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