The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Rational Design of MOF/COF Hybrid Materials for Photocatalytic H2 Evolution in the Presence of Sacrificial Electron Donors
Abstract
Crystalline and porous covalent organic frameworks (COFs) and metal‐organic frameworks (MOFs) materials have attracted enormous attention in the field of photocatalytic H 2 evolution due to their long‐range order structures, large surface areas, outstanding visible light absorbance, and tunable band gaps. In this work, we successfully integrated two‐dimensional (2D) COF with stable MOF. By covalently anchoring NH 2‐UiO‐66 onto the surface of TpPa‐1‐COF, a new type of MOF/COF hybrid materials with high surface area, porous framework, and high crystallinity was synthesized. The resulting hierarchical porous hybrid materials show efficient photocatalytic H 2 evolution under visible light irradiation. Especially, NH 2‐UiO‐66/TpPa‐1‐COF (4:6) exhibits the maximum photocatalytic H 2 evolution rate of 23.41 mmol g−1 h−1 (with the TOF of 402.36 h−1), which is approximately 20 times higher than that of the parent TpPa‐1‐COF and the best performance photocatalyst for H 2 evolution among various MOF‐ and COF‐based photocatalysts.
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Citations
Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Cited by
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Xu, M., Li, D., Sun, K., Jiao, L., Xie, C., Ding, C., & Jiang, H. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202104219 · Cited by 280
Liu, S., Wang, M., He, Y., Cheng, Q., Qian, T., & Yan, C. (2023) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2022.214882 · Cited by 236
Metadata
- Authors
- Zhang, F., Sheng, J., Yang, Z., Sun, X., Tang, H., Lu, M., Dong, H., Shen, F., Liu, J., & Lan, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-08-07
- Volume
- 57
- Issue
- 37
- Pages
- 12106-12110
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2884922654
- Cited by
- 719
- References
- 1
- FWCI
- 14.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, F., Sheng, J., Yang, Z., Sun, X., Tang, H., Lu, M., Dong, H., Shen, F., Liu, J., & Lan, Y. (2018). Rational Design of MOF/COF Hybrid Materials for Photocatalytic H2 Evolution in the Presence of Sacrificial Electron Donors. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201806862
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