The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
The Radical Pathway Based on a Lithium‐Metal‐Compatible High‐Dielectric Electrolyte for Lithium–Sulfur Batteries
Abstract
High‐dielectric solvents were explored for enhancing the sulfur utilization in lithium–sulfur (Li−S) batteries, but their applications have been impeded by low stability at the lithium metal anode. Now a radical‐directed, lithium‐compatible, and strongly polysulfide‐solvating high‐dielectric electrolyte based on tetramethylurea is presented. Over 200 hours of cycling was realized in Li|Li symmetric cells, showing good compatibility of the tetramethylurea‐based electrolyte with lithium metal. The high solubility of short‐chain polysulfides, as well as the presence of active S 3.− radicals, enabled pouch cells to deliver a discharge capacity of 1524 mAh g−1 and an energy density of 324 Wh kg−1. This finding suggests an alternative recipe to ether‐based electrolytes for Li−S batteries.
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Citations
Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Cited by
Hou, L.-P., Zhang, X.-Q., Li, B.-Q., & Zhang, Q. (2021) · Materials Today · doi:10.1016/j.mattod.2020.10.021 · Cited by 283
Self-citationToward Practical High‐Energy‐Density Lithium–Sulfur Pouch Cells: A Review
Chen, Z., Zhao, M., Hou, L., Zhang, X., Li, B., & Huang, J. (2022) · Advanced Materials · doi:10.1002/adma.202201555 · Cited by 282
Self-citationCathode Kinetics Evaluation in Lean-Electrolyte Lithium–Sulfur Batteries
Chen, Z.-X., Cheng, Q., Li, X.-Y., Li, Z., Song, Y.-W., Sun, F., Zhao, M., Zhang, X.-Q., Li, B.-Q., & Huang, J.-Q. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.3c02786 · Cited by 279
Self-citationExploring and Understanding the Roles of Li2Sn and the Strategies to beyond Present Li-S Batteries
Lei, J., Liu, T., Chen, J., Zheng, M., Zhang, Q., Mao, B., & Dong, Q. (2020) · Chem · doi:10.1016/j.chempr.2020.06.032 · Cited by 268
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Metadata
- Authors
- Zhang, G., Peng, H., Zhao, C., Chen, X., Zhao, L., Li, P., Huang, J., & Zhang, Q.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-11-26
- Volume
- 57
- Issue
- 51
- Pages
- 16732-16736
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2899446056
- Cited by
- 243
- References
- 1
- FWCI
- 9.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, G., Peng, H., Zhao, C., Chen, X., Zhao, L., Li, P., Huang, J., & Zhang, Q. (2018). The Radical Pathway Based on a Lithium‐Metal‐Compatible High‐Dielectric Electrolyte for Lithium–Sulfur Batteries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201810132
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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