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Nickel Metal–Organic Framework Monolayers for Photoreduction of Diluted CO2: Metal‐Node‐Dependent Activity and Selectivity
Abstract
Photocatalytic conversion of diluted CO 2 into solar fuel is highly appealing yet still in its infancy. Herein, we demonstrate the metal‐node‐dependent performance for photoreduction of diluted CO 2 by constructing Ni metal–organic framework (MOF) monolayers (Ni MOLs). In diluted CO 2 (10 %), Ni MOLs exhibit a highest apparent quantum yield of 1.96 % with a CO selectivity of 96.8 %, which not only exceeds reported systems in diluted CO 2 but also is superior to most catalysts in pure CO 2. Whereas isostructural Co MOLs is almost inactive in diluted CO 2, indicating the performance is dependent on the metal nodes. Experimental and theoretical investigations show that strong CO 2 binding affinity of Ni MOLs is the crucial factor, which stabilizes the Ni‐CO 2 adducts and facilitates CO 2‐to‐CO conversion.
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Citations
Cites
Future CO 2 Emissions and Climate Change from Existing Energy Infrastructure
Davis, S. J., Caldeira, K., & Matthews, H. D. (2010) · Science · doi:10.1126/science.1188566 · Cited by 1,399
Cited by
Carbon capture and conversion using metal–organic frameworks and MOF-based materials
Ding, M., Flaig, R. W., Jiang, H.-L., & Yaghi, O. M. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00829a · Cited by 2,616
Product selectivity of photocatalytic CO2 reduction reactions
Fu, J., Jiang, K., Qiu, X., Yu, J., & Liu, M. (2020) · Materials Today · doi:10.1016/j.mattod.2019.06.009 · Cited by 1,280
Wang, L., Chen, W., Zhang, D., Du, Y., Amal, R., Qiao, S., Wu, J., & Yin, Z. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00163h · Cited by 905
Zhong, W., Sa, R., Li, L., He, Y., Li, L., Bi, J., Zhuang, Z., Yu, Y., & Zou, Z. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b02997 · Cited by 769
Powerful combination of MOFs and C3N4 for enhanced photocatalytic performance
Wang, C.-C., Yi, X.-H., & Wang, P. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.01.091 · Cited by 419
Metadata
- Authors
- Han, B., Ou, X., Deng, Z., Song, Y., Tian, C., Deng, H., Xu, Y., & Lin, Z.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-11-21
- Volume
- 57
- Issue
- 51
- Pages
- 16811-16815
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2899684319
- Cited by
- 529
- References
- 1
- FWCI
- 12.33
- Type
- journal article
- Language
- en
- Open access
- closed
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- Han, B., Ou, X., Deng, Z., Song, Y., Tian, C., Deng, H., Xu, Y., & Lin, Z. (2018). Nickel Metal–Organic Framework Monolayers for Photoreduction of Diluted CO2: Metal‐Node‐Dependent Activity and Selectivity. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201811545
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