The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Ultrathin Nitrogen‐Doped Holey Carbon@Graphene Bifunctional Electrocatalyst for Oxygen Reduction and Evolution Reactions in Alkaline and Acidic Media
Abstract
Efficient nonprecious‐metal oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) electrocatalysts are key for the commercial viability of fuel cells, metal–air batteries, and water‐splitting systems. Thus, high‐performance ORR and OER electrocatalysts in acidic electrolytes are needed to support high‐efficiency proton exchange membrane (PEM)‐based systems. Herein, we report a new approach to design and prepare an ultrathin N‐doped holey carbon layer (HCL) on a graphene sheet that exhibits outstanding bifunctional ORR/OER activities in both alkaline and acidic media. The edge sites of HCL are utilized to achieve selective doping of highly active pyridinic‐N. The sandwiched graphene sheet provides mechanical support, stabilizes HCL structure and promotes charge transfer. The synergetic effect of the catalyst structure overcomes the drawbacks of holey graphene approaches. The resulting ORR and OER performances are equal to or better than the top‐ranked electrocatalysts.
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Cites
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Zhong, H., Wang, J., Zhang, Y., Xu, W., Xing, W., Xu, D., Zhang, Y., & Zhang, X. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201408990 · Cited by 938
Cited by
Yuan, K., Lützenkirchen-Hecht, D., Li, L., Shuai, L., Li, Y., Cao, R., Qiu, M., Zhuang, X., Leung, M. K. H., Chen, Y., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b11852 · Cited by 1,047
Zhao, C., Liu, J., Li, B., Ren, D., Chen, X., Yu, J., & Zhang, Q. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202003619 · Cited by 641
Rong, C., Dastafkan, K., Wang, Y., & Zhao, C. (2023) · Advanced Materials · doi:10.1002/adma.202211884 · Cited by 361
Self-citationSingle-site pyrrolic-nitrogen-doped sp2-hybridized carbon materials and their pseudocapacitance
Tian, K., Wang, J., Cao, L., Yang, W., Guo, W., Liu, S., Li, W., Wang, F., Li, X., Xu, Z., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-17727-y · Cited by 319
Advances in Oxygen Evolution Electrocatalysts for Proton Exchange Membrane Water Electrolyzers
Chen, Z., Guo, L., Pan, L., Yan, T., He, Z., Li, Y., Shi, C., Huang, Z., Zhang, X., & Zou, J. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202103670 · Cited by 298
Metadata
- Authors
- Sun, J., Lowe, S. E., Zhang, L., Wang, Y., Pang, K., Wang, Y., Zhong, Y., Liu, P., Zhao, K., Tang, Z., & Zhao, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-11-14
- Volume
- 57
- Issue
- 50
- Pages
- 16511-16515
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2898902949
- Cited by
- 349
- References
- 2
- FWCI
- 9.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sun, J., Lowe, S. E., Zhang, L., Wang, Y., Pang, K., Wang, Y., Zhong, Y., Liu, P., Zhao, K., Tang, Z., & Zhao, H. (2018). Ultrathin Nitrogen‐Doped Holey Carbon@Graphene Bifunctional Electrocatalyst for Oxygen Reduction and Evolution Reactions in Alkaline and Acidic Media. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201811573
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