The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Carbon‐Supported Divacancy‐Anchored Platinum Single‐Atom Electrocatalysts with Superhigh Pt Utilization for the Oxygen Reduction Reaction
Abstract
Maximizing the platinum utilization in electrocatalysts toward oxygen reduction reaction (ORR) is very desirable for large‐scale sustainable application of Pt in energy systems. A cost‐effective carbon‐supported carbon‐defect‐anchored platinum single‐atom electrocatalysts (Pt 1/C) with remarkable ORR performance is reported. An acidic H 2/O 2 single cell with Pt 1/C as cathode delivers a maximum power density of 520 mW cm−2 at 80 °C, corresponding to a superhigh platinum utilization of 0.09 g Pt kW−1. Further physical characterization and density functional theory computations reveal that single Pt atoms anchored stably by four carbon atoms in carbon divacancies (Pt‐C 4) are the main active centers for the observed high ORR performance.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
Nørskov, J. K., Rossmeisl, J., Logadottir, A., Lindqvist, L., Kitchin, J. R., Bligaard, T., & Jónsson, H. (2004) · The Journal of Physical Chemistry B · doi:10.1021/jp047349j · Cited by 13,153
A fast and robust algorithm for Bader decomposition of charge density
Henkelman, G., Arnaldsson, A., & Jónsson, H. (2006) · Computational Materials Science · doi:10.1016/j.commatsci.2005.04.010 · Cited by 10,723
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Self-citationHigh performance platinum single atom electrocatalyst for oxygen reduction reaction
Liu, J., Jiao, M., Lu, L., Barkholtz, H. M., Li, Y., Wang, Y., Jiang, L., Wu, Z., Liu, D.-J., Zhuang, L., et al. (2017) · Nature Communications · doi:10.1038/ncomms15938 · Cited by 772
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Cited by
Single atom electrocatalysts supported on graphene or graphene-like carbons
Fei, H., Dong, J., Chen, D., Hu, T., Duan, X., Shakir, I., Huang, Y., & Duan, X. (2019) · Chemical Society Reviews · doi:10.1039/c9cs00422j · Cited by 673
Recent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Liu, B., Feng, R., Busch, M., Wang, S., Wu, H., Liu, P., Gu, J., Bahadoran, A., Matsumura, D., Tsuji, T., et al. (2022) · ACS Nano · doi:10.1021/acsnano.2c04077 · Cited by 143
Yang, Z., Chen, C., Zhao, Y., Wang, Q., Zhao, J., Waterhouse, G. I. N., Qin, Y., Shang, L., & Zhang, T. (2023) · Advanced Materials · doi:10.1002/adma.202208799 · Cited by 120
Metadata
- Authors
- Liu, J., Jiao, M., Mei, B., Tong, Y., Li, Y., Ruan, M., Song, P., Sun, G., Jiang, L., Wang, Y., Jiang, Z., Gu, L., Zhou, Z., & Xu, W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-12-20
- Volume
- 58
- Issue
- 4
- Pages
- 1163-1167
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2904124880
- Cited by
- 340
- References
- 4
- FWCI
- 8.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, J., Jiao, M., Mei, B., Tong, Y., Li, Y., Ruan, M., Song, P., Sun, G., Jiang, L., Wang, Y., Jiang, Z., Gu, L., Zhou, Z., & Xu, W. (2019). Carbon‐Supported Divacancy‐Anchored Platinum Single‐Atom Electrocatalysts with Superhigh Pt Utilization for the Oxygen Reduction Reaction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201812423
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