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Highly Reversible and Rechargeable Safe Zn Batteries Based on a Triethyl Phosphate Electrolyte
Abstract
Zinc metal is an attractive anode material for next‐generation batteries. However, dendrite growth and limited Coulombic efficiency (CE) during cycling are the major roadblocks towards the widespread commercialization of batteries employing Zn anodes. In this work we report the novel adoption of triethyl phosphate (TEP) as a solvent and co‐solvent with aqueous electrolytes to obtain a highly stable and dendrite‐free Zn anode. Stable Zn plating/stripping for over 3000 h was obtained, accompanied by a CE of 99.68 %. SEM images of the Zn anodes revealed highly porous interconnected dendrite‐free Zn deposits. The electrolyte displayed good compatibility with both Zn anodes and potassium copper hexacyanoferrate (KCuHCf) cathodes for Zn ion batteries (ZIBs). The full cell showed a long cycling stability and high rate capability. The present work is a contribution towards cost‐effective and safe battery systems.
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Citations
Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Liu, S., Zhu, H., Zhang, B., Li, G., Zhu, H., Ren, Y., Geng, H., Yang, Y., Liu, Q., & Li, C. C. (2020) · Advanced Materials · doi:10.1002/adma.202001113 · Cited by 561
Zeng, X., Xie, K., Liu, S., Zhang, S., Hao, J., Liu, J., Pang, W. K., Liu, J., Rao, P., Wang, Q., et al. (2021) · Energy & Environmental Science · doi:10.1039/d1ee01851e · Cited by 528
Insight on Organic Molecules in Aqueous Zn‐Ion Batteries with an Emphasis on the Zn Anode Regulation
Wang, D., Li, Q., Zhao, Y., Hong, H., Li, H., Huang, Z., Liang, G., Yang, Q., & Zhi, C. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202102707 · Cited by 478
Design of a Solid Electrolyte Interphase for Aqueous Zn Batteries
Li, D., Cao, L., Deng, T., Liu, S., & Wang, C. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202103390 · Cited by 466
Metadata
- Authors
- Naveed, A., Yang, H., Yang, J., Nuli, Y., & Wang, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-01-25
- Volume
- 58
- Issue
- 9
- Pages
- 2760-2764
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2906901660
- Cited by
- 530
- References
- 0
- FWCI
- 24.06
- Type
- journal article
- Language
- en
- Open access
- closed
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- Naveed, A., Yang, H., Yang, J., Nuli, Y., & Wang, J. (2019). Highly Reversible and Rechargeable Safe Zn Batteries Based on a Triethyl Phosphate Electrolyte. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201813223
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