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Metal–Organic Frameworks with Target‐Specific Active Sites Switched by Photoresponsive Motifs: Efficient Adsorbents for Tailorable CO2 Capture
Abstract
Photoresponsive metal–organic frameworks (PMOFs) are of interest for tailorable CO 2 adsorption. However, modulation of CO 2 adsorption on PMOFs is based on steric hindrance or structural change owing to weak interactions between CO 2 and active sites. It is challenging to fabricate PMOFs with strong but tailorable sites for CO 2 adsorption. Now, the construction of PMOFs with target‐specific (strong) active sites is achieved by introducing tetraethylenepentamine into azobenzene‐functionalized MOFs for tailorable CO 2 adsorption. Amines are specific active sites for CO 2, contributing to capture CO 2 selectively. Cis/trans isomerization of azobenzene motifs trigged by UV/Vis light adjusts the electrostatic potential of amines significantly, leading to exposure/shelter of amines and modulation of CO 2 adsorption on strong active sites. This system enables us to design adsorption processes for CO 2 capture from mixtures, which is impossible to realize by traditional PMOFs.
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Cites
Carbon capture and storage: how green can black be
Haszeldine, R. S. (2009) · Science · doi:10.1126/science.1172246 · Cited by 2,021
An overview of CO2 capture technologies
MacDowell, N., Florin, N., Buchard, A., Hallett, J., Galindo, A., Jackson, G., Adjiman, C. S., Williams, C. K., Shah, N., & Fennell, P. (2010) · Energy & Environmental Science · doi:10.1039/c004106h · Cited by 1,636
Cited by
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Recent advances in carbon capture storage and utilisation technologies: a review
Osman, A. I., Hefny, M., Abdel Maksoud, M. I. A., Elgarahy, A. M., & Rooney, D. W. (2021) · Environmental Chemistry Letters · doi:10.1007/s10311-020-01133-3 · Cited by 862
Porous organic polymers for CO2capture, separation and conversion
Song, K. S., Fritz, P. W., & Coskun, A. (2022) · Chemical Society Reviews · doi:10.1039/d2cs00727d · Cited by 409
Chemically modified carbonaceous adsorbents for enhanced CO2 capture: A review
Kamran, U., & Park, S.-J. (2021) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2020.125776 · Cited by 262
Carbon Capture Technologies: A Review on Technology Readiness Level
Hekmatmehr, H., Esmaeili, A., Pourmahdi, M., Atashrouz, S., Abedi, A., Ali Abuswer, M., Nedeljkovic, D., Latifi, M., Farag, S., & Mohaddespour, A. (2024) · Fuel · doi:10.1016/j.fuel.2024.130898 · Cited by 189
Metadata
- Authors
- Jiang, Y., Tan, P., Qi, S., Liu, X., Yan, J., Fan, F., & Sun, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-02-21
- Volume
- 58
- Issue
- 20
- Pages
- 6600-6604
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2912145129
- Cited by
- 217
- References
- 2
- FWCI
- 10.45
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jiang, Y., Tan, P., Qi, S., Liu, X., Yan, J., Fan, F., & Sun, L. (2019). Metal–Organic Frameworks with Target‐Specific Active Sites Switched by Photoresponsive Motifs: Efficient Adsorbents for Tailorable CO2 Capture. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201900141
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