The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Isolated Diatomic Ni‐Fe Metal–Nitrogen Sites for Synergistic Electroreduction of CO2
Open accessAbstract
Polynary single‐atom structures can combine the advantages of homogeneous and heterogeneous catalysts while providing synergistic functions based on different molecules and their interfaces. However, the fabrication and identification of such an active‐site prototype remain elusive. Here we report isolated diatomic Ni‐Fe sites anchored on nitrogenated carbon as an efficient electrocatalyst for CO 2 reduction. The catalyst exhibits high selectivity with CO Faradaic efficiency above 90 % over a wide potential range from −0.5 to −0.9 V (98 % at −0.7 V), and robust durability, retaining 99 % of its initial selectivity after 30 hours of electrolysis. Density functional theory studies reveal that the neighboring Ni‐Fe centers not only function in synergy to decrease the reaction barrier for the formation of COOH* and desorption of CO, but also undergo distinct structural evolution into a CO‐adsorbed moiety upon CO 2 uptake.
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Cites
Atomically dispersed Ni(i) as the active site for electrochemical CO2 reduction
Yang, H. B., Hung, S.-F., Liu, S., Yuan, K., Miao, S., Zhang, L., Huang, X., Wang, H.-Y., Cai, W., Chen, R., et al. (2018) · Nature Energy · doi:10.1038/s41560-017-0078-8 · Cited by 2,239
Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Recent Advances in Inorganic Heterogeneous Electrocatalysts for Reduction of Carbon Dioxide
Zhu, D. D., Liu, J. L., & Qiao, S. Z. (2016) · Advanced Materials · doi:10.1002/adma.201504766 · Cited by 1,594
Competition between CO 2 Reduction and H 2 Evolution on Transition-Metal Electrocatalysts
Zhang, Y.-J., Sethuraman, V., Michalsky, R., & Peterson, A. A. (2014) · ACS Catalysis · doi:10.1021/cs5012298 · Cited by 509
Trends in electrochemical CO2 reduction activity for open and close-packed metal surfaces
Shi, C., Hansen, H. A., Lausche, A. C., & Nørskov, J. K. (2014) · Physical Chemistry Chemical Physics · doi:10.1039/c3cp54822h · Cited by 465
Cited by
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
Wang, G., Chen, J., Ding, Y., Cai, P., Yi, L., Li, Y., Tu, C., Hou, Y., Wen, Z., & Dai, L. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00071j · Cited by 1,295
Emerging Dual‐Atomic‐Site Catalysts for Efficient Energy Catalysis
Zhang, W., Chao, Y., Zhang, W., Zhou, J., Lv, F., Wang, K., Lin, F., Luo, H., Li, J., Tong, M., et al. (2021) · Advanced Materials · doi:10.1002/adma.202102576 · Cited by 528
Self-citationRong, C., Shen, X., Wang, Y., Thomsen, L., Zhao, T., Li, Y., Lu, X., Amal, R., & Zhao, C. (2022) · Advanced Materials · doi:10.1002/adma.202110103 · Cited by 503
Self-citationJiao, L., Yang, W., Wan, G., Zhang, R., Zheng, X., Zhou, H., Yu, S., & Jiang, H. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202008787 · Cited by 412
Self-citationWang, P., Ren, Y., Wang, R., Zhang, P., Ding, M., Li, C., Zhao, D., Qian, Z., Zhang, Z., Zhang, L., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-15416-4 · Cited by 394
Metadata
- Authors
- Ren, W., Tan, X., Yang, W., Jia, C., Xu, S., Wang, K., Smith, S. C., & Zhao, C.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-04-17
- Volume
- 58
- Issue
- 21
- Pages
- 6972-6976
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2933816311
- Cited by
- 1,036
- References
- 5
- FWCI
- 25.30
- Type
- journal article
- Language
- en
- Open access
- green
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- Ren, W., Tan, X., Yang, W., Jia, C., Xu, S., Wang, K., Smith, S. C., & Zhao, C. (2019). Isolated Diatomic Ni‐Fe Metal–Nitrogen Sites for Synergistic Electroreduction of CO2. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201901575
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