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Lithium Chlorides and Bromides as Promising Solid‐State Chemistries for Fast Ion Conductors with Good Electrochemical Stability
Abstract
Enabling all‐solid‐state Li‐ion batteries requires solid electrolytes with high Li ionic conductivity and good electrochemical stability. Following recent experimental reports of Li 3 YCl 6 and Li 3 YBr 6 as promising new solid electrolytes, we used first principles computation to investigate the Li‐ion diffusion, electrochemical stability, and interface stability of chloride and bromide materials and elucidated the origin of their high ionic conductivities and good electrochemical stabilities. Chloride and bromide chemistries intrinsically exhibit low migration energy barriers, wide electrochemical windows, and are not constrained to previous design principles for sulfide and oxide Li‐ion conductors, allowing for much greater freedom in structure, chemistry, composition, and Li sublattice for developing fast Li‐ion conductors. Our study highlights chloride and bromide chemistries as a promising new research direction for solid electrolytes with high ionic conductivity and good stability.
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Cited by
Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes
Banerjee, A., Wang, X., Fang, C., Wu, E. A., & Meng, Y. S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00101 · Cited by 1,526
Tan, D. H. S., Banerjee, A., Chen, Z., & Meng, Y. S. (2020) · Nature Nanotechnology · doi:10.1038/s41565-020-0657-x · Cited by 641
Site-Occupation-Tuned Superionic LixScCl3+xHalide Solid Electrolytes for All-Solid-State Batteries
Liang, J., Li, X., Wang, S., Adair, K. R., Li, W., Zhao, Y., Wang, C., Hu, Y., Zhang, L., Zhao, S., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00134 · Cited by 567
Self-citationWang, C., Liang, J., Zhao, Y., Zheng, M., Li, X., & Sun, X. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00551k · Cited by 489
Kwak, H., Wang, S., Park, J., Liu, Y., Kim, K. T., Choi, Y., Mo, Y., & Jung, Y. S. (2022) · ACS Energy Letters · doi:10.1021/acsenergylett.2c00438 · Cited by 341
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Metadata
- Authors
- Wang, S., Bai, Q., Nolan, A. M., Liu, Y., Gong, S., Sun, Q., & Mo, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-05-15
- Volume
- 58
- Issue
- 24
- Pages
- 8039-8043
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2936895644
- Cited by
- 654
- References
- 6
- FWCI
- 17.18
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, S., Bai, Q., Nolan, A. M., Liu, Y., Gong, S., Sun, Q., & Mo, Y. (2019). Lithium Chlorides and Bromides as Promising Solid‐State Chemistries for Fast Ion Conductors with Good Electrochemical Stability. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201901938
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