The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Generating Defect‐Rich Bismuth for Enhancing the Rate of Nitrogen Electroreduction to Ammonia
Abstract
The electrochemical N 2 fixation, which is far from practical application in aqueous solution under ambient conditions, is extremely challenging and requires a rational design of electrocatalytic centers. We observed that bismuth (Bi) might be a promising candidate for this task because of its weak binding with H adatoms, which increases the selectivity and production rate. Furthermore, we successfully synthesized defect‐rich Bi nanoplates as an efficient noble‐metal‐free N 2 reduction electrocatalyst via a low‐temperature plasma bombardment approach. When exclusively using 1 H NMR measurements with N 2 gas as a quantitative testing method, the defect‐rich Bi(110) nanoplates achieved a 15 NH 3 production rate of 5.453 μg mg Bi−1 h−1 and a Faradaic efficiency of 11.68 % at −0.6 V vs. RHE in aqueous solution at ambient conditions.
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Opportunities and challenges for a sustainable energy future
Chu, S., & Majumdar, A. (2012) · Nature · doi:10.1038/nature11475 · Cited by 12,550
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
Greeley, J., Jaramillo, T. F., Bonde, J., Chorkendorff, I., & Nørskov, J. K. (2006) · Nature Materials · doi:10.1038/nmat1752 · Cited by 4,097
Montoya, J. H., Tsai, C., Vojvodic, A., & Nørskov, J. K. (2015) · ChemSusChem · doi:10.1002/cssc.201500322 · Cited by 1,384
Cited by
Guo, X., Gu, J., Lin, S., Zhang, S., Chen, Z., & Huang, S. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b13349 · Cited by 1,151
Self-citationRen, Y., Yu, C., Tan, X., Huang, H., Wei, Q., & Qiu, J. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03596c · Cited by 565
Comprehensive Understanding of the Thriving Ambient Electrochemical Nitrogen Reduction Reaction
Zhao, X., Hu, G., Chen, G., Zhang, H., Zhang, S., & Wang, H. (2021) · Advanced Materials · doi:10.1002/adma.202007650 · Cited by 503
Greatly Improving Electrochemical N 2 Reduction over TiO 2 Nanoparticles by Iron Doping
Wu, T., Zhu, X., Xing, Z., Mou, S., Li, C., Qiao, Y., Liu, Q., Luo, Y., Shi, X., Zhang, Y., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201911153 · Cited by 499
Self-citationGuo, Y., Zhang, R., Zhang, S., Zhao, Y., Yang, Q., Huang, Z., Dong, B., & Zhi, C. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00806d · Cited by 498
Metadata
- Authors
- Wang, Y., Shi, M., Bao, D., Meng, F., Zhang, Q., Zhou, Y., Liu, K., Zhang, Y., Wang, J., Chen, Z., Liu, D., Jiang, Z., Luo, M., Gu, L., Zhang, Q., Cao, X., Yao, Y., Shao, M., Zhang, Y., Zhang, X., Chen, J. G., Yan, J., & Jiang, Q.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-05-30
- Volume
- 58
- Issue
- 28
- Pages
- 9464-9469
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2946633992
- Cited by
- 278
- References
- 4
- FWCI
- 10.12
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Y., Shi, M., Bao, D., Meng, F., Zhang, Q., Zhou, Y., Liu, K., Zhang, Y., Wang, J., Chen, Z., Liu, D., Jiang, Z., Luo, M., Gu, L., Zhang, Q., Cao, X., Yao, Y., Shao, M., Zhang, Y., . . . Jiang, Q. (2019). Generating Defect‐Rich Bismuth for Enhancing the Rate of Nitrogen Electroreduction to Ammonia. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201903969
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