The DOI matches its Crossref record; 70 of the 70 references it cites were found in a registry or an index.
Three‐Phase Photocatalysis for the Enhanced Selectivity and Activity of CO2 Reduction on a Hydrophobic Surface
Open accessAbstract
The photocatalytic CO 2 reduction reaction (CRR) represents a promising route for the clean utilization of stranded renewable resources, but poor selectivity resulting from the competing hydrogen evolution reaction (HER) in aqueous solution limits its practical applicability. In the present contribution a photocatalyst with hydrophobic surfaces was fabricated. It facilitates an efficient three‐phase contact of CO 2 (gas), H 2 O (liquid), and catalyst (solid). Thus, concentrated CO 2 molecules in the gas phase contact the catalyst surface directly, and can overcome the mass‐transfer limitations of CO 2, inhibit the HER because of lowering proton contacts, and overall enhance the CRR. Even when loaded with platinum nanoparticles, one of the most efficient HER promotion cocatalysts, the three‐phase photocatalyst maintains a selectivity of 87.9 %. Overall, three‐phase photocatalysis provides a general and reliable method to enhance the competitiveness of the CRR.
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Wagner, A., Sahm, C. D., & Reisner, E. (2020) · Nature Catalysis · doi:10.1038/s41929-020-00512-x · Cited by 731
Z‐Scheme Photocatalytic Systems for Carbon Dioxide Reduction: Where Are We Now?
Zhang, W., Mohamed, A. R., & Ong, W. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201914925 · Cited by 667
Rare‐Earth Single Erbium Atoms for Enhanced Photocatalytic CO2 Reduction
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Metadata
- Authors
- Li, A., Cao, Q., Zhou, G., Schmidt, B. V. K. J., Zhu, W., Yuan, X., Huo, H., Gong, J., & Antonietti, M.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-09-04
- Volume
- 58
- Issue
- 41
- Pages
- 14549-14555
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2968693108
- Cited by
- 403
- References
- 70
- FWCI
- 9.22
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Li, A., Cao, Q., Zhou, G., Schmidt, B. V. K. J., Zhu, W., Yuan, X., Huo, H., Gong, J., & Antonietti, M. (2019). Three‐Phase Photocatalysis for the Enhanced Selectivity and Activity of CO2 Reduction on a Hydrophobic Surface. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201908058
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