The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Graphitic Carbon Nitride (g‐C3N4): An Interface Enabler for Solid‐State Lithium Metal Batteries
Abstract
Solid‐state Li metal batteries (SSLMBs) have attracted considerable interests due to their promising energy density as well as high safety. However, the realization of a well‐matched Li metal/solid‐state electrolyte (SSE) interface remains challenging. Herein, we report g‐C 3 N 4 as a new interface enabler. We discover that introducing g‐C 3 N 4 into Li metal can not only convert the Li metal/garnet‐type SSE interface from point contact to intimate contact but also greatly enhance the capability to suppress the dendritic Li formation because of the greatly enhanced viscosity, decreased surface tension of molten Li, and the in situ formation of Li 3 N at the interface. Thus, the resulting Li‐C 3 N 4|SSE|Li‐C 3 N 4 symmetric cell gives a significantly low interfacial resistance of 11 Ω cm 2 and a high critical current density (CCD) of 1500 μA cm−2. In contrast, the same symmetric cell configuration with pristine Li metal electrodes has a much larger interfacial resistance (428 Ω cm 2) and a much lower CCD (50 μA cm−2).
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Jain, A., Ong, S. P., Hautier, G., Chen, W., Richards, W. D., Dacek, S., Cholia, S., Gunter, D., Skinner, D., Ceder, G., et al. (2013) · APL Materials · doi:10.1063/1.4812323 · Cited by 13,094
Serial Block-Face Scanning Electron Microscopy to Reconstruct Three-Dimensional Tissue Nanostructure
Denk, W., & Horstmann, H. (2004) · PLoS Biology · doi:10.1371/journal.pbio.0020329 · Cited by 1,644
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Physicochemical Concepts of the Lithium Metal Anode in Solid-State Batteries
Krauskopf, T., Richter, F. H., Zeier, W. G., & Janek, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00431 · Cited by 892
Reducing the thickness of solid-state electrolyte membranes for high-energy lithium batteries
Wu, J., Yuan, L., Zhang, W., Li, Z., Xie, X., & Huang, Y. (2021) · Energy & Environmental Science · doi:10.1039/d0ee02241a · Cited by 425
Self-citationThe nonmetal modulation of composition and morphology of g-C3N4-based photocatalysts
He, F., Wang, Z., Li, Y., Peng, S., & Liu, B. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.118828 · Cited by 346
Self-citationElectrolyte/Electrode Interfaces in All-Solid-State Lithium Batteries: A Review
Pang, Y., Pan, J., Yang, J., Zheng, S., & Wang, C. (2021) · Electrochemical Energy Reviews · doi:10.1007/s41918-020-00092-1 · Cited by 313
Zhao, F., Sun, Q., Yu, C., Zhang, S., Adair, K., Wang, S., Liu, Y., Zhao, Y., Liang, J., Wang, C., et al. (2020) · ACS Energy Letters · doi:10.1021/acsenergylett.0c00207 · Cited by 294
Metadata
- Authors
- Huang, Y., Chen, B., Duan, J., Yang, F., Wang, T., Wang, Z., Yang, W., Hu, C., Luo, W., & Huang, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-01-29
- Volume
- 59
- Issue
- 9
- Pages
- 3699-3704
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3003479500
- Cited by
- 295
- References
- 2
- FWCI
- 14.19
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, Y., Chen, B., Duan, J., Yang, F., Wang, T., Wang, Z., Yang, W., Hu, C., Luo, W., & Huang, Y. (2020). Graphitic Carbon Nitride (g‐C3N4): An Interface Enabler for Solid‐State Lithium Metal Batteries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201914417
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