The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
Designing Atomic Active Centers for Hydrogen Evolution Electrocatalysts
Abstract
The evolution of hydrogen from water using renewable electrical energy is a topic of current interest. Pt/C exhibits the highest catalytic activity for the H 2 evolution reaction (HER), but scarce supplies and high cost limit its large‐scale application. Atomic active centers in single‐atom catalysts, single‐atom alloys, and catalysts with two atom sorts exhibit maximum atomic efficiency, unique structure, and exceptional activity for the HER. Interactions between well‐defined active sites and supports are known to affect electron transfer and dramatically accelerate the reaction. This Review first highlights methods for studying atomic active centers for the HER. Then, active sites with different coordination configurations are described. Active centers with one metal atom, two different metal atoms as well as nonmetal atoms are analyzed at the atomic scale. Finally, future research perspectives are proposed.
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Citations
Cites
Noble metal-free hydrogen evolution catalysts for water splitting
Zou, X., & Zhang, Y. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00448e · Cited by 5,955
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
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Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li + -Ni(OH) 2 -Pt Interfaces
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Nanostructured hydrotreating catalysts for electrochemical hydrogen evolution
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Hydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Platinum single-atom and cluster catalysis of the hydrogen evolution reaction
Cheng, N., Stambula, S., Wang, D., Banis, M. N., Liu, J., Riese, A., Xiao, B., Li, R., Sham, T.-K., Liu, L.-M., et al. (2016) · Nature Communications · doi:10.1038/ncomms13638 · Cited by 2,072
Self-citationAtomic cobalt on nitrogen-doped graphene for hydrogen generation
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Catalysis by Supported Single Metal Atoms
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Cited by
Electrocatalysis of Single-Atom Sites: Impacts of Atomic Coordination
Lu, B., Liu, Q., & Chen, S. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c01950 · Cited by 394
Wang, Y., Liu, Y., Liu, W., Wu, J., Li, Q., Feng, Q., Chen, Z., Xiong, X., Wang, D., & Lei, Y. (2020) · Energy & Environmental Science · doi:10.1039/d0ee02833a · Cited by 303
Self-citationTheoretical Advances in Understanding and Designing the Active Sites for Hydrogen Evolution Reaction
Sun, F., Tang, Q., & Jiang, D.-E. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c02081 · Cited by 285
Liu, R., Gong, Z., Liu, J., Dong, J., Liao, J., Liu, H., Huang, H., Liu, J., Yan, M., Huang, K., et al. (2021) · Advanced Materials · doi:10.1002/adma.202103533 · Cited by 152
Han, Y., Duan, H., Liu, W., Zhou, C., Wang, B., Jiang, Q., Feng, S., Yan, W., Tan, T., & Zhang, R. (2023) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2023.122898 · Cited by 80
Metadata
- Authors
- Lei, Y., Wang, Y., Liu, Y., Song, C., Li, Q., Wang, D., & Li, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-09-02
- Volume
- 59
- Issue
- 47
- Pages
- 20794-20812
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3000644301
- Cited by
- 387
- References
- 31
- FWCI
- 12.38
- Type
- journal article
- Language
- en
- Open access
- closed
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