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Ultrathin ZnIn2S4 Nanosheets Anchored on Ti3C2TX MXene for Photocatalytic H2 Evolution
Abstract
Photocatalysts derived from semiconductor heterojunctions that harvest solar energy and catalyze reactions still suffer from low solar‐to‐hydrogen conversion efficiency. Now, MXene (Ti 3 C 2 T X) nanosheets (MNs) are used to support the in situ growth of ultrathin ZnIn 2 S 4 nanosheets (UZNs), producing sandwich‐like hierarchical heterostructures (UZNs‐MNs‐UZNs) for efficient photocatalytic H 2 evolution. Opportune lateral epitaxy of UZNs on the surface of MNs improves specific surface area, pore diameter, and hydrophilicity of the resulting materials, all of which could be beneficial to the photocatalytic activity. Owing to the Schottky junction and ultrathin 2D structures of UZNs and MNs, the heterostructures could effectively suppress photoexcited electron–hole recombination and boost photoexcited charge transfer and separation. The heterostructure photocatalyst exhibits improved photocatalytic H 2 evolution performance (6.6 times higher than pristine ZnIn 2 S 4) and excellent stability.
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Wang, Q., Hisatomi, T., Jia, Q., Tokudome, H., Zhong, M., Wang, C., Pan, Z., Takata, T., Nakabayashi, M., Shibata, N., et al. (2016) · Nature Materials · doi:10.1038/nmat4589 · Cited by 1,684
Cited by
Surface Modification of 2D Photocatalysts for Solar Energy Conversion
Feng, C., Wu, Z., Huang, K., Ye, J., & Zhang, H. (2022) · Advanced Materials · doi:10.1002/adma.202200180 · Cited by 456
Tan, M., Ma, Y., Yu, C., Luan, Q., Li, J., Liu, C., Dong, W., Su, Y., Qiao, L., Gao, L., et al. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202111740 · Cited by 394
Self-citationEmerging Cocatalysts on g‐C3N4 for Photocatalytic Hydrogen Evolution
Zhu, Q., Xu, Z., Qiu, B., Xing, M., & Zhang, J. (2021) · Small · doi:10.1002/smll.202101070 · Cited by 380
Metadata
- Authors
- Zuo, G., Wang, Y., Teo, W. L., Xie, A., Guo, Y., Dai, Y., Zhou, W., Jana, D., Xian, Q., Dong, W., & Zhao, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-05-07
- Volume
- 59
- Issue
- 28
- Pages
- 11287-11292
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3014345698
- Cited by
- 603
- References
- 1
- FWCI
- 19.32
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zuo, G., Wang, Y., Teo, W. L., Xie, A., Guo, Y., Dai, Y., Zhou, W., Jana, D., Xian, Q., Dong, W., & Zhao, Y. (2020). Ultrathin ZnIn2S4 Nanosheets Anchored on Ti3C2TX MXene for Photocatalytic H2 Evolution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202002136
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