Cited by 198Electrocatalysts for Energy Conversion2D Materials and ApplicationsMetalloenzymes and iron-sulfur proteins

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Distance Synergy of MoS2‐Confined Rhodium Atoms for Highly Efficient Hydrogen Evolution

Meng, Xiangyu, Ma, Chao, Jiang, Luozhen, Si, Rui, Meng, Xianguang, Tu, Yunchuan, Yu, Liang, Bao, Xinhe, Deng, Dehui·2020·Angewandte Chemie International Edition

DOI 10.1002/anie.202003484

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Abstract

Perturbing the electronic structure of the MoS 2 basal plane by confining heteroatoms offers the opportunity to trigger in‐plane activity for the hydrogen evolution reaction (HER). The key challenge consists of inducing the optimum HER activity by controlling the type and distribution of confined atoms. A distance synergy of MoS 2‐confined single‐atom rhodium is presented, leading to an ultra‐high HER activity at the in‐plane S sites adjacent to the rhodium. By optimizing the distance between the confined Rh atoms, an ultra‐low overpotential of 67 mV is achieved at a current density of 10 mA cm−2 in acidic solution. Experiments and first‐principles calculations demonstrate a unique distance synergy between the confined rhodium atoms in tuning the reactivity of neighboring in‐plane S atoms, which presents a volcanic trend with the inter‐rhodium distance. This study provides a new strategy to tailor the activity of MoS 2 surface via modulating the distance between confined single atoms.

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Ehsan, M., Akilarasan, M., Hakeem, A., Ahmed, B., Ahmed, S., Patel, F., Farooq, W., Tahir, M. N., & Gondal, M. A. (2026) · International journal of hydrogen energy · doi:10.1016/j.ijhydene.2026.155138
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Authors: Meng, X., Ma, C., Jiang, L., Si, R., Meng, X., Tu, Y., Yu, L., Bao, X., & Deng, D.
Affiliations: Dalian Institute of Chemical Physics (CN)
Hunan University (CN)
Chinese Academy of Sciences (CN)
Corresponding author: Yu, Liang
Deng, Dehui
ORCID: Meng, Xiangyu
Ma, Chao
Si, Rui
Meng, Xianguang
Tu, Yunchuan
Yu, Liang
Bao, Xinhe
Deng, Dehui
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2020-04-30
Volume: 59
Issue: 26
Pages: 10502-10507
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.202003484
OpenAlex: W3013511951
Cited by: 198
References: 0
Citations by year: 2026: 25 · 2025: 31 · 2024: 28 · 2023: 31 · 2022: 44 · 2021: 32 · 2020: 7
FWCI: 5.63
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Funders: the National Key R&D Program of China (No. 2016YFA0204100 and 2016YFA0200200)
the National Natural Science Foundation of China (No. 21890753 and 21988101, No. 21872140)
the Key Research Program of Frontier Sciences of the Chinese Academy of Sciences (No. QYZDB-SSW-JSC020)
the DNL Cooperation Fund, CAS (No. DNL180201)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
Life Sciences › Biochemistry, Genetics and Molecular Biology › Biochemistry › Metalloenzymes and iron-sulfur proteins
Keywords: MoS2, single-atom catalysts, rhodium, hydrogen evolution reaction, electronic structure modulation, volcano plot, acidic electrocatalysis, overpotential

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Distance Synergy of MoS2‐Confined Rhodium Atoms for Highly Efficient Hydrogen Evolution

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