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Holey Lamellar High‐Entropy Oxide as an Ultra‐High‐Activity Heterogeneous Catalyst for Solvent‐free Aerobic Oxidation of Benzyl Alcohol
Open accessAbstract
The development of noble‐metal‐free heterogeneous catalysts is promising for selective oxidation of aromatic alcohols; however, the relatively low conversion of non‐noble metal catalysts under solvent‐free atmospheric conditions hinders their industrial application. Now, a holey lamellar high entropy oxide (HEO) Co 0.2 Ni 0.2 Cu 0.2 Mg 0.2 Zn 0.2 O material with mesoporous structure is prepared by an anchoring and merging process. The HEO has ultra‐high catalytic activity for the solvent‐free aerobic oxidation of benzyl alcohol. Up to 98 % conversion can be achieved in only 2 h, to our knowledge, the highest conversion of benzyl alcohol by oxidation to date. By regulating the catalytic reaction parameters, benzoic acid or benzaldehyde can be selectively optimized as the main product. Analytical characterizations and calculations provide a deeper insight into the catalysis mechanism, revealing abundant oxygen vacancies and holey lamellar framework contribute to the ultra‐high catalytic activity.
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Cites
Nanocrystal Growth on Graphene with Various Degrees of Oxidation
Wang, H., Robinson, J. T., Diankov, G., & Dai, H. (2010) · Journal of the American Chemical Society · doi:10.1021/ja100329d · Cited by 530
Cited by
High-entropy materials for catalysis: A new frontier
Sun, Y., & Dai, S. (2021) · Science Advances · doi:10.1126/sciadv.abg1600 · Cited by 942
Self-citationUnderstanding the Role of Entropy in High Entropy Oxides
Aamlid, S. S., Oudah, M., Rottler, J., & Hallas, A. M. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.2c11608 · Cited by 574
High-entropy alloys in electrocatalysis: from fundamentals to applications
Ren, J.-T., Chen, L., Wang, H.-Y., & Yuan, Z.-Y. (2023) · Chemical Society Reviews · doi:10.1039/d3cs00557g · Cited by 551
High-entropy materials for energy and electronic applications
Schweidler, S., Botros, M., Strauss, F., Wang, Q., Ma, Y., Velasco, L., Cadilha Marques, G., Sarkar, A., Kübel, C., Hahn, H., et al. (2024) · Nature Reviews Materials · doi:10.1038/s41578-024-00654-5 · Cited by 448
High‐Entropy Atomic Layers of Transition‐Metal Carbides (MXenes)
Du, Z., Wu, C., Chen, Y., Cao, Z., Hu, R., Zhang, Y., Gu, J., Cui, Y., Chen, H., Shi, Y., et al. (2021) · Advanced Materials · doi:10.1002/adma.202101473 · Cited by 322
Metadata
- Authors
- Feng, D., Dong, Y., Zhang, L., Ge, X., Zhang, W., Dai, S., & Qiao, Z.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-06-30
- Volume
- 59
- Issue
- 44
- Pages
- 19503-19509
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W3029312876
- Cited by
- 272
- References
- 1
- FWCI
- 12.23
- Type
- journal article
- Language
- en
- Open access
- green
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- Feng, D., Dong, Y., Zhang, L., Ge, X., Zhang, W., Dai, S., & Qiao, Z. (2020). Holey Lamellar High‐Entropy Oxide as an Ultra‐High‐Activity Heterogeneous Catalyst for Solvent‐free Aerobic Oxidation of Benzyl Alcohol. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202004892
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